Spontaneous fission modes and lifetimes of super-heavy elements in the nuclear density functional theory
arXiv:1208.1215 · doi:10.1103/PhysRevC.87.024320
Abstract
Lifetimes of super-heavy (SH) nuclei are primarily governed by alpha decay and spontaneous fission (SF). Here we study the competing decay modes of even-even SH isotopes with 108 <= Z <= 126 and 148 <= N <= 188 using the state-of-the-art self-consistent nuclear density functional theory framework capable of describing the competition between nuclear attraction and electrostatic repulsion. The collective mass tensor of the fissioning superfluid nucleus is computed by means of the cranking approximation to the adiabatic time-dependent Hartree-Fock-Bogoliubov approach. Along the path to fission, our calculations allow for the simultaneous breaking of axial and space inversion symmetries; this may result in lowering SF lifetimes by more than seven orders of magnitude in some cases. We predict two competing SF modes: reflection-symmetric and reflection-asymmetric.The shortest-lived SH isotopes decay by SF; they are expected to lie in a narrow corridor formed by Hs, Fl, and Uuo that separates the regions of SH nuclei synthesized in "cold fusion" and "hot fusion" reactions. The region of long-lived SH nuclei is expected to be centered on Ds with a total half-life of ?1.5 days.
6 pages, 4 figures
References in corpus (9)
- Fission half-lives of super-heavy nuclei in a microscopic approach
- Fission barriers in covariant density functional theory: extrapolation to superheavy nuclei
- Microscopic description of complex nuclear decay: multimodal fission
- Fission modes of mercury isotopes
- Relativistic Energy Density Functional Description of Shape Transition in Superheavy Nuclei
- Pairing renormalization and regularization within the local density approximation
- Superdeformed Oblate Superheavy Nuclei?
- Nuclear fission with mean-field instantons
- Collective inertia and fission barriers within the Skyrme-Hartree-Fock theory
Cited by in corpus (78)
- Microscopic Theory of Nuclear Fission: A Review
- Review on the progress in nuclear fission
- Formation and dynamics of fission fragments
- Multidimensionally-constrained relativistic mean field models and potential energy surfaces of actinide nuclei
- r-Process Nucleosynthesis: Connecting Rare-Isotope Beam Facilities with the Cosmos
- Fission fragment charge and mass distributions in 239Pu(n,f) in the adiabatic nuclear energy density functional theory
- Octupole deformation in the ground states of even-even nuclei: a global analysis within the covariant density functional theory
- Multidimensionally-constrained covariant density functional theories --- nuclear shapes and potential energy surfaces
- Description of Induced Nuclear Fission with Skyrme Energy Functionals: I. Static Potential Energy Surfaces and Fission Fragment Properties
- Theory of Nuclear Fission
- Fission barriers and probabilities of spontaneous fission for elements with Z100
- Pairing-induced speedup of nuclear spontaneous fission
- Dissipative dynamics in quasi-fission
- Covariant density functional theory: Reexamining the structure of superheavy nuclei
- Fission properties of superheavy nuclei for r-process calculations
- Microscopic modeling of mass and charge distributions in the spontaneous fission of 240Pu
- Properties of heaviest nuclei with and
- Multidimensionally-constrained relativistic mean-field study of spontaneous fission: coupling between shape and pairing degrees of freedom
- Dynamic versus static fission paths with realistic interactions
- Spontaneous fission lifetimes from the minimization of self-consistent collective action
- The many facets of the (non relativistic) Nuclear Equation of State
- Microscopic study of induced fission dynamics of Th with covariant energy density functionals
- Microscopic description of fission in Uranium isotopes with the Gogny energy density functional
- Shape evolution and collective dynamics of quasifission in TDHF
- Adiabatic fission barriers in superheavy nuclei
- Cluster Radioactivity in Super Heavy Nuclei
- Assessing theoretical uncertainties in fission barriers of superheavy nuclei
- Recoil-alpha-fission and recoil-alpha-alpha-fission events observed in the reaction Ca-48 + Am-243
- Third minima in thorium and uranium isotopes in a self-consistent theory
- Cluster radioactivity of Og
- Fission properties of the BCPM functional
- Symmetry energy in nuclear density functional theory
- Time-dependent HF approach to SHE dynamics
- Formation and distribution of fragments in the spontaneous fission of 240Pu
- Isotopic trends of quasifission and fusion-fission in the reactions Ca+Pu
- Spontaneous fission of superheavy nucleus Fl
- An experimental survey of the production of alpha decaying heavy elements in the reactions of U +Th at 7.5-6.1 MeV/nucleon
- Microscopic description of fission in superheavy nuclei with the parametrization D1M of the Gogny energy density functional
- Constraining the surface properties of effective Skyrme interactions
- Thermal fission rates with temperature dependent fission barriers
- Structure of Superheavy Nuclei Along Element 115 Decay Chains
- Toroidal high-spin isomers in the nucleus
- Fission decay of Cn studied using cranking inertia
- Two-body dissipation effects on synthesis of superheavy elements
- Global calculations on the microscopic energies and nuclear deformations: Isospin dependence of the spin-orbit coupling
- Feasibility of observing the α decay chains from isotopes of SHN with Z = 128, Z = 126, Z = 124 and Z = 122
- Microscopic description of fission in odd-mass uranium and plutonium nuclei with the Gogny energy density functional
- Description of the multidimensional potential energy surface in fission of Cf and No
- Least action description of spontaneous fission in fermium and nobelium nuclei based on the Gogny energy density functional
- Microscopic description of fission in nobelium isotopes with the Gogny-D1M energy density functional
- Folded potentials in cluster physics - a comparison of Yukawa and Coulomb potentials with Riesz fractional integrals
- Microscopic description of the self-conjugate Xe and Te -decay chain
- Potential energy surfaces and fission fragment mass yields of even-even superheavy nuclei
- Neural Network Emulation of Spontaneous Fission
- A dynamical model calculation to reconcile the nuclear fission lifetime from different measurement techniques
- Isotopic yield in cold binary fission of even-even Cf isotopes
- Scission configuration in the self-consistent calculations with neck constraint
- Fission barriers of two odd-neutron actinide nuclei taking into account the time-reversal symmetry breaking at the mean-field level
- Microscopic model for the collective enhancement of nuclear level densities
- Predictions on the alpha decay chains of superheavy nuclei with Z =121 within the range 290 A 339
- Global analysis of Skyrme forces with higher-order density dependence
- Density Functional Theory with Spatial-Symmetry Breaking and Configuration Mixing
- Least action description of dynamic pairing correlations in the fission of Curium and Californium isotopes based on the Gogny energy density functional
- A microscopic model for spontaneous fission: validity of the adiabatic approximation
- Superfluid fission dynamics with microscopic approaches
- Nuclear fission in covariant density functional theory
- Ground state and fission properties of even- uranium isotopes from multidimensionally-constrained relativistic mean field model
- Structural and decay properties of nuclei appearing in the -decay chains of 120 within the relativistic mean-field formalism
- A novel experimental setup for rare events selection and its potential application to super heavy elements search
- Fusion-fission probabilities, cross sections and structure notes of super-heavy nuclei
- Microscopic description of spontaneous fission based on a Gogny energy density functional including tensor contributions
- Theoretical studies on structural properties and decay modes of 119 isotopes
- Multimodal fission from self-consistent calculations
- FRIB and the GW170817 Kilonova
- The role of the Heisenberg principle in Constrained Molecular Dynamics model
- Shell plus pairing effect arguments for cluster preformation at the nuclear surface in cold fission
- Microscopic pairing in fission dynamics
- Microscopic Theory of Nuclear Fission