Collective Plasmonic-Molecular Modes in the Strong Coupling Regime
arXiv:1201.2151 · doi:10.1103/PhysRevLett.109.073002
Abstract
We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling strength grows, a new mode emerges, which is attributed to long range molecular interactions mediated by the plasmonic field. The new, molecular-like mode repels the polariton states, and leads to an opening of energy gaps both below and above the asymptotic free molecule energy.
8 pages, 6 figures, submitted to PRL
References in corpus (8)
- Theory of extraordinary optical transmission through subwavelength hole arrays
- Vacuum Rabi splitting and strong coupling dynamics for surface plasmon polaritons and Rhodamine 6G molecules
- Coherent coupling between surface plasmons and excitons in semiconductor nanocrystals
- Strong coupling between a metallic nanoparticle and a single molecule
- Ultra strong coupling regime and plasmon-polaritons in parabolic semiconductor quantum wells
- Cooperative emission of light by an ensemble of dipoles near a metal nanostucture: The plasmonic Dicke effect
- Strong coupling of localized plasmons and molecular excitons in nanostructured silver films
- Numerical studies of the interaction of an atomic sample with the electromagnetic field in two dimensions
Cited by in corpus (34)
- Strong coupling between surface plasmon polaritons and emitters
- Theory of the strong coupling between quantum emitters and propagating surface plasmons
- Transformation Optics Approach to Plasmon-Exciton Strong Coupling in Nanocavities
- Topical Review: optics of exciton-plasmon nanomaterials
- Plexcitons: Dirac points and topological modes
- Origin of the asymmetric light emission from molecular exciton-polaritons
- Manipulating the Interaction between Localized and Delocalized Surface Plasmon Polaritons in Graphene
- Ultrafast Energy Transfer Between Molecular Assemblies and Surface Plasmons in the Strong Coupling Regime
- Spontaneous decay of a quantum emitter near a plasmonic nanostructure
- Tailoring optical response of a hybrid comprising a quantum dimer emitter strongly coupled to a metal nanoparticle
- Exciton-plasmon energy exchange drives the transition to strong coupling regime
- Stimulated Raman Adiabatic Passage (STIRAP) as a Route to Achieving Optical Control in Plasmonics
- Molecular nanoplasmonics: self-consistent electrodynamics in current carrying junctions
- Plasmon-induced coherence, exciton-induced transparency and Fano interference for hybrid plasmonic systems in strong coupling regime
- Exciton-induced transparency in hybrid plasmonic systems
- Theory of Dipole Induced Electromagnetic Transparency
- Molecular plasmonics: the role of ro-vibrational molecular states in exciton-plasmon materials under strong coupling conditions
- Non-Hermitian wave packet approximation of Bloch optical equations
- Surface plasmon-polaritons in periodic arrays of V-grooves strongly coupled to quantum emitters
- Quantum emitter dipole-dipole interactions in nanoplasmonic systems
- Nanoporous Metallic Network as a Largescale 3D Source of Second Harmonic Light
- Control of optical properties of hybrid materials with chirped femtosecond laser pulses under strong coupling conditions
- Exciton-plasmaritons in graphene-semiconductor structures
- Cooperative emission mediated by cooperative energy transfer to a plasmonic antenna
- Non-Markovian effects for hybrid plasmonic systems in the strong coupling regime
- Optical absorption spectroscopy in hybrid systems of plasmons and excitons
- Inverse design of broadband, strongly-coupled plexcitonic nonlinear metasurfaces
- Universal optical polarizability for plasmonic nanostructures
- Area theorem for surface plasmons interacting with resonant atoms
- Second Harmonic Generation from a Single Plasmonic Nanorod Strongly Coupled to a WSe2 Monolayer
- Space Quantization of Light Transmission by Strong Coupling of Plasmonic Cavity Modes with Photosynthetic Complexes
- Strong coupling regime in coherent electron transport in periodic quantum nanostructures
- Observation of Strong Coupling between an Inverse Bowtie Nano-Antenna and a Single J-aggregate
- Efficient DNA-driven nanocavities for approaching quasi-deterministic strong coupling to a few fluorophores