Spin Waves and magnetic exchange interactions in insulating Rb$_{0.89}$Fe$_{1.58}$Se$_2$

Miaoyin Wang; Chen Fang; Dao-Xin Yao; GuoTai Tan; Leland W. Harriger; Yu Song; Tucker Netherton; Chenglin Zhang; Meng Wang; Matthew B. Stone; Wei Tian; Jiangping Hu; Pengcheng Dai

doi:10.1038/ncomms1573

paper

Spin Waves and magnetic exchange interactions in insulating Rb $_{0.89}$ Fe $_{1.58}$ Se $_{2}$

arXiv:1105.4675 · doi:10.1038/ncomms1573

Abstract

The discovery of alkaline iron selenide $A$ Fe $_{1.6 + x}$ Se $_{2}$ ( $A =$ K, Rb, Cs) superconductors has generated considerable excitement in the condensed matter physics community because superconductivity in these materials may have a different origin from the sign reversed s-wave electron pairing mechanism, a leading candidate proposed for all other Fe-based superconductors. Although $A$ Fe $_{1.6 + x}$ Se $_{2}$ are isostructural with the metallic antiferromagnetic (AF) iron pnictides such as (Ba,Ca,Sr)Fe $_{2}$ As $_{2}$ , they are insulators near $x = 0$ and form a $5 \times 5$ blocked AF structure (Fig. 1a) completely different from the iron pnictides. If magnetism is responsible for superconductivity of all iron-based materials, it is important to determine their common magnetic features. Here we use neutron scattering to map out spin waves in the AF insulating Rb $_{0.89}$ Fe $_{1.58}$ Se $_{2}$ . We find that although Rb $_{0.89}$ Fe $_{1.58}$ Se $_{2}$ has a N $e ˊ$ el temperature ( $T_{N} = 475$ K) much higher than that of the iron pnictides ( $T_{N} \leq 220$ K), spin waves for both classes of materials have similar zone boundary energies. A comparison of the fitted effective exchange couplings using a local moment Heisenberg Hamiltonian in Rb $_{0.89}$ Fe $_{1.58}$ Se $_{2}$ , (Ba,Ca,Sr)Fe $_{2}$ As $_{2}$ , and iron chalcogenide Fe $_{1.05}$ Te reveals that their next nearest neighbor (NNN) exchange couplings are similar. Therefore, superconductivity in all Fe-based materials may have a common magnetic origin that is intimately associated with the NNN magnetic exchange interactions, even though they have metallic or insulating ground states, different AF orders and electronic band structures.

13 pages, 9 figures

Spin Waves and magnetic exchange interactions in insulating Rb $_{0.89}$ Fe $_{1.58}$ Se $_{2}$

Abstract

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Spin Waves and magnetic exchange interactions in insulating Rb0.89​Fe1.58​Se2​

Abstract

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Cited by in corpus (68)

Spin Waves and magnetic exchange interactions in insulating Rb $_{0.89}$ Fe $_{1.58}$ Se $_{2}$