activity
19962025
most citedTheoretical evidence for a dense fluid precursor to crystallization

229 citations · 1.9k across the 71 of their papers we have counts for

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35 papers · 1 filter

cond-mat.stat-mech2025

Approximate calculation of multidimensional first passage times

James F. Lutsko

The general, multidimensional barrier crossing problem for diffusive processes under the action of conservative forces is studied with the goal of developing tractable approximatio…

cond-mat.stat-mech2025

The use of open boundaries in stochastic hydrodynamic models of nucleation

James F. Lutsko

Stochastic hydrodynamics is a central tool in the study of first order phase transitions at a fundamental level. Combined with sophisticated free energy models, e.g. as developed i…

cond-mat.stat-mech2021★ 7 cited

Classical Density Functional Theory in the Canonical Ensemble

James F. Lutsko

Classical density functional theory for finite temperatures is usually formulated in the grand-canonical ensemble where arbitrary variations of the local density are possible. Howe…

cond-mat.stat-mech2020★ 25 cited

Explicitly stable Fundamental Measure Theory models for classical density functional theory

James F. Lutsko

The derivation of the state of the art tensorial versions of Fundamental Measure Theory (a form of classical Density Functional Theory for hard spheres) are re-examined in the ligh…

cond-mat.stat-mech2020★ 6 cited

Long-wavelength density fluctuations as nucleation precursors

James F. Lutsko, Julien Lam

Recent theories of nucleation that go beyond Classical Nucleation Theory predict that diffusion-limited nucleation of both liquid droplets and of crystals from a low-density vapor…

cond-mat.stat-mech2016

Temporal Fokker-Planck Equations

Jean Pierre Boon, James F. Lutsko

The temporal Fokker-Plank equation [{\it J. Stat. Phys.}, {\bf 3/4}, 527 (2003)] or propagation-dispersion equation was derived to describe diffusive processes with temporal disper…

cond-mat.stat-mech2014★ 5 cited

Molecular theory of anomalous diffusion - Application to Fluorescence Correlation Spectroscopy

Jean Pierre Boon, James F. Lutsko

The nonlinear theory of anomalous diffusion is based on particle interactions giving an explicit microscopic description of diffusive processes leading to sub-, normal, or super-di…

cond-mat.stat-mech2014

New comments on "Possible divergences in Tsallis' thermostatistics''

James F. Lutsko, Jean Pierre Boon

In a recent letter ({\it{EPL}}, {\bf{104}} (2013) 60003; see also {\it {arXiv:1309.5645}}), Plastino and Rocca suggest that the divergences inherent to the formulation of nonextens…

cond-mat.stat-mech2013

Comment on "Possible divergences in Tsallis' thermostatistics"

Jean Pierre Boon, James F. Lutsko

The problematic divergence of the -partition function of the harmonic oscillator recently considered in \cite{plastino} is a particular case of the non-normalizabilty of the dis…

cond-mat.stat-mech2013★ 25 cited

Molecular theory of anomalous diffusion

James F. Lutsko, Jean Pierre Boon

We present a Master Equation formulation based on a Markovian random walk model that exhibits sub-diffusion, classical diffusion and super-diffusion as a function of a single param…

cond-mat.stat-mech2012★ 5 cited

Direct correlation function from the consistent fundamental-measure free energies for hard-sphere mixtures

James F. Lutsko

In a recent publication[PRE 86, 04012 (2012)], Santos has presented a self-consistency condition that can be used to limit the possible forms of Fundamental Measure Theory. Here, t…

cond-mat.stat-mech2011★ 26 cited

A microscopic approach to nonlinear Reaction-Diffusion: the case of morphogen gradient formation

Jean Pierre Boon, James F. Lutsko, Christopher Lutsko

We develop a microscopic theory for reaction-difusion (R-D) processes based on a generalization of Einstein's master equation with a reactive term and we show how the mean field fo…

cond-mat.stat-mech2011★ 22 cited

Questioning the validity of non-extensive thermodynamics for classical Hamiltonian systems

J. F. Lutsko, J. P. Boon

We examine the non-extensive approach to the statistical mechanics of Hamiltonian systems with where is the classical kinetic energy. Our analysis starts from the basic…

cond-mat.stat-mech2010★ 5 cited

The low-density/high-density liquid phase transition for model globular proteins

Patrick Grosfils, James F. Lutsko

The effect of molecule size (excluded volume) and the range of interaction on the surface tension, phase diagram and nucleation properties of a model globular protein is investigat…

cond-mat.stat-mech2010

Is nonextensive statistics applicable to continuous Hamiltonian systems?

J. P. Boon, J. F. Lutsko

The homogeneous entropy for continuous systems in nonextensive statistics reads , where is the phase space variable. O…

cond-mat.stat-mech2009★ 29 cited

Is the Tsallis entropy stable?

James F. Lutsko, Jean Pierre Boon, Patrick Grosfils

The question of whether the Tsallis entropy is Lesche-stable is revisited. It is argued that when physical averages are computed with the escort probabilities, the correct applicat…

cond-mat.stat-mech2008★ 52 cited

Density Functional Theory of Inhomogeneous Liquids: III. Liquid-Vapor Nucleation

James F. Lutsko

The process of nucleation of vapor bubbles from a superheated liquid and of liquid droplets from a supersaturated vapor is investigated using the Modified-Core van der Waals model…

cond-mat.stat-mech2008★ 27 cited

Theoretical description of the nucleation of vapor bubbles in a superheated fluid

James F. Lutsko

The nucleation of vapor bubbles within a superheated fluid is studied using density functional theory. The nudged elastic band technique is used to find the minimum energy pathway…

cond-mat.stat-mech2008★ 54 cited

Dependence of the liquid-vapor surface tension on the range of interaction: a test of the law of corresponding states

Patrick Grosfils, James F. Lutsko

The planar surface tension of coexisting liquid and vapor phases of a fluid of Lennard-Jones atoms is studied as a function of the range of the potential using both Monte Carlo sim…

cond-mat.stat-mech2008★ 32 cited

Density Functional Theory of Inhomogeneous Liquids: II. A Fundamental Measure Approach

James F. Lutsko

Previously, it has been shown that the direct correlation function for a Lennard-Jones fluid could be modeled by a sum of that for hard-spheres, a mean-field tail and a simple line…

cond-mat.stat-mech2007★ 27 cited

Generalized Diffusion

James F. Lutsko, Jean Pierre Boon

The Fokker-Planck equation for the probability to find a random walker at position at time is derived for the case that the the probability to make jumps depends n…

cond-mat.stat-mech2007★ 24 cited

Density functional theory of inhomogeneous liquids. I. The liquid-vapor interface in Lennard-Jones fluids

James F. Lutsko

A simple model is proposed for the direct correlation function (DCF) for simple fluids consisting of a hard-core contribution, a simple parametrized core correction, and a mean-fie…

cond-mat.stat-mech2007★ 19 cited

Nonlinear diffusion from Einstein's master equation

J. P. Boon, J. F. Lutsko

We generalize Einstein's master equation for random walk processes by considering that the probability for a particle at position to make a jump of length lattice sites, $P…

cond-mat.stat-mech2006★ 19 cited

Properties of non-FCC hard-sphere solids predicted by density functional theory

James F. Lutsko

The free energies of the FCC, BCC, HCP and Simple Cubic phases for hard spheres are calculated as a function of density using the Fundamental Measure Theory models of Rosenfeld et…