activity
19962025
most citedTheoretical evidence for a dense fluid precursor to crystallization

229 citations · 1.9k across the 71 of their papers we have counts for

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23 papers · 1 filter

cond-mat.soft2024

COLIS: an advanced light scattering apparatus for investigating the structure and dynamics of soft matter onboard the International Space Station

Alessandro Martinelli, Stefano Buzzaccaro, Quentin Galand +8

Colloidal Solids (COLIS) is a state-of-the-art light scattering setup developed for experiments onboard the International Space Station (ISS). COLIS allows for probing the structur…

cond-mat.soft2021★ 5 cited

Reconsidering Power Functional Theory

James F. Lutsko, Martin Oettel

The original derivation of Power Functional Theory, Schmidt and Brader, JCP 138, 214101 (2013), is reworked in some detail with a view to clarifying and simplifying the logic and m…

cond-mat.soft2018★ 11 cited

Solvent-mediated interactions between nanostructures: from water to Lennard-Jones liquid

Julien Lam, James F. Lutsko

Solvent-mediated interactions emerge from complex mechanisms that depend on the solute structure, its wetting properties and the nature of the liquid. While numerous studies have f…

cond-mat.soft2018★ 42 cited

Classical density functional theory, unconstrained crystallization, and polymorphic behavior

James F. Lutsko, Julien Lam

While in principle, finite temperature density functional theory (ftDFT) should be a powerful tool for the study of crystallization, in practice this has not so far been the case.…

cond-mat.soft2018★ 11 cited

Solute particle near a nanopore: influence of size and surface properties on the solvent-mediated forces

Julien Lam, James F. Lutsko

Nanoscopic pores are used in various systems to attract nanoparticles. In general the behaviour is a result of two types of interactions: the material specific affinity and the sol…

cond-mat.soft2018★ 13 cited

Lattice induced crystallization of nanodroplets: the role of finite-size effects and substrate properties in controlling polymorphism

Julien Lam, James F. Lutsko

Targeting specific technological applications requires the control of nanoparticle properties, especially the crystalline polymorph. Freezing a nanodroplet deposited on a solid sub…

cond-mat.soft2016

Mechanism for the stabilization of protein clusters above the solubility curve

James F. Lutsko, Grégoire Nicolis

Pan, Vekilov and Lubchenko[\textit{J. Phys. Chem. B}, 2010, \textbf{114}, 7620] have proposed that dense stable protein clusters appearing in weak protein solutions above the solub…

cond-mat.soft2015★ 2 cited

Unification of classical nucleation theories via unified Itô-Stratonovich stochastic equation

Miguel A. Durán-Olivencia, James F. Lutsko

Classical nucleation theory (CNT) is the most widely used framework to describe the early stage of first-order phase transitions. Unfortunately the different points of view adopted…

cond-mat.soft2014★ 17 cited

Extending classical nucleation theory to confined systems

Miguel A. Durán-Olivencia, James F. Lutsko

Classical nucleation theory has been recently reformulated based on fluctuating hydrodynamics [J.F. Lutsko and M.A. Durán-Olivencia, J. Chem. Phys. 138, 244908 (2013)]. The present…

cond-mat.soft2012★ 11 cited

Nucleation of colloids and macromolecules in a finite volume

James F. Lutsko

A recently formulated description of homogeneous nucleation for Brownian particles in the over-damped limit based on fluctuating hydrodynamics is used to determine the nucleation p…

cond-mat.soft2012★ 10 cited

Nucleation of colloids and macromolecules: does the nucleation pathway matter?

James F. Lutsko

A recent description of diffusion-limited nucleation based on fluctuating hydrodynamics that extends classical nucleation theory predicts a very non-classical two-step scenario whe…

cond-mat.soft2011★ 90 cited

A dynamical theory of nucleation for colloids and macromolecules

James F. Lutsko

A general theory of nucleation for colloids and macromolecules in solution is formulated within the context of fluctuating hydrodynamics. A formalism for the determination of nucle…

cond-mat.soft2011★ 30 cited

A dynamical theory of homogeneous nucleation for colloids and macromolecules

James F. Lutsko

Homogeneous nucleation is formulated within the context of fluctuating hydrodynamics. It is shown that for a colloidal or macromolecular system in the strong damping limit the most…

cond-mat.soft2011

On the role of metastable intermediate states in the homogeneous nucleation of solids from solution

James F. Lutsko

The role of metastable liquid phases in vapor-crystal nucleation is studied using Density Functional Theory(DFT). The model gives a semi-quantitatively accurate description of both…

cond-mat.soft2011★ 48 cited

Density Functional Theory of Inhomogeneous Liquids IV. Squared-gradient approximation and Classical Nucleation Theory

James F. Lutsko

The Squared-Gradient approximation to the Modified-Core Van der Waals density functional theory model is developed. A simple, explicit expression for the SGA coefficient involving…

cond-mat.soft2010★ 8 cited

Kinetic roughening-like transition with finite nucleation barrier

James F. Lutsko, Vasileios Basios, Gregoire Nicolis +3

Recent observations of the growth of protein crystals have identified two different growth regimes. At low supersaturation, the surface of the crystal is smooth and increasing in s…

cond-mat.soft2005★ 1 cited

Hydrodynamics of an inelastic gas with implications for sonochemistry

James F. Lutsko

The hydrodynamics for a gas of hard-spheres which sometimes experience inelastic collisions resulting in the loss of a fixed, velocity-independent, amount of energy is investig…

cond-mat.soft2005★ 89 cited

Transport properties of dense dissipitive hard-sphere fluids for arbitrary energy loss models

James F. Lutsko

The revised Enskog approximation for a fluid of hard spheres which lose energy upon collision is discussed for the case that the energy is lost from the normal component of the vel…

cond-mat.soft2004★ 52 cited

The rheology of dense, polydisperse granular fluids under shear

James F. Lutsko

The solution of the Enskog equation for the one-body velocity distribution of a moderately dense, arbitrary mixture of inelastic hard spheres undergoing planar shear flow is descri…

cond-mat.soft2004

Spontaneous development of 3-D structure in sheared granular flows

James F. Lutsko

Computer simulations of sheared granular fluids, modeled as inelastic hard spheres, are presented which show signs of a uniquely three-dimensional instabilty. In the stable regime,…

cond-mat.soft2002★ 58 cited

Diffusion in a Granular Fluid - Simulation

James Lutsko, J. Javier Brey, James W. Dufty

The linear response description for impurity diffusion in a granular fluid undergoing homogeneous cooling is developed in the preceeding paper. The formally exact Einstein and Gree…

cond-mat.soft2002★ 48 cited

Diffusion in a Granular Fluid - Theory

James W. Dufty, J. Javier Brey, James Lutsko

Many important properties of granular fluids can be represented by a system of hard spheres with inelastic collisions. Traditional methods of nonequilibrium statistical mechanics a…

cond-mat.soft2000★ 64 cited

A model for the atomic-scale structure of a dense, nonequilibrium fluid: the homogeneous cooling state of granular fluids

James F. Lutsko

It is shown that the equilibrium Generalized Mean Spherical Model of fluid structure may be extended to nonequilibrium states with equation of state information used in equilibrium…