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quant-ph2025
Rotational excitation of molecules in the regime of strong ro-vibrational coupling: Comparison between an optical centrifuge and a transform-limited pulse
J. M. García-Garrido, V. Milner, C. P. Koch +1
We investigate theoretically the ability of an optical centrifuge - a laser pulse whose linear polarization is rotating at an accelerated rate, to control molecular rotation in the…
quant-ph2025
Control of molecular rotation in helium nanodroplets with an optical centrifuge
Ian MacPhail-Bartley, Alexander A. Milner, Frank Stienkemeier +1
We experimentally demonstrate that the rotation of molecules embedded in helium nanodroplets can be controlled with an optical centrifuge, allowing for the study of molecular dynam…