activity
20072026
most citedControl of molecular rotation with a chiral train of ultrashort pulses

84 citations · 365 across the 18 of their papers we have counts for

collaborators

19 papers

cond-mat.mtrl-sci2026

Ultrafast Magnetization Induced from Raman-Active Axial Chiral Phonons

Chuankun Huang, Alexander Milner, Jiaming Luo +8

Axial chiral phonons, which carry angular momentum and exhibit unusually large magnetic moments, provide a new degree of freedom for controlling the time-reversal symmetry and magn…

quant-ph2026

Optical centrifuge as a probe of strong dissipative coupling between a molecular rotor and superfluid helium

Ian MacPhail-Bartley, Sören E. Mahr, Cameron E. Peters +7

A macroscopic manifestation of superfluidity is that objects moving through liquid helium experience negligible friction below the Landau critical velocity. How this frictionless m…

cond-mat.other2026

Coherent spectroscopy of collective excitations in superfluid helium far from equilibrium

Gabriel Voith, Alexander A. Milner, Michael J. Desrochers +2

Ultrafast dynamics of collective excitations in superfluids remains largely unexplored beyond the roton region of the Landau excitation spectrum, despite the importance of such dyn…

quant-ph2025

Rotational excitation of molecules in the regime of strong ro-vibrational coupling: Comparison between an optical centrifuge and a transform-limited pulse

J. M. García-Garrido, V. Milner, C. P. Koch +1

We investigate theoretically the ability of an optical centrifuge - a laser pulse whose linear polarization is rotating at an accelerated rate, to control molecular rotation in the…

physics.chem-ph2025

Ultraslow optical centrifuge with arbitrarily low rotational acceleration

Kevin Wang, Ian MacPhail-Bartley, Cameron E. Peters +1

We outline the design and characterization of a laser pulse shaper, which creates an ``ultraslow optical centrifuge'' - a linearly polarized field whose polarization vector rotates…

quant-ph2025

Control of molecular rotation in helium nanodroplets with an optical centrifuge

Ian MacPhail-Bartley, Alexander A. Milner, Frank Stienkemeier +1

We experimentally demonstrate that the rotation of molecules embedded in helium nanodroplets can be controlled with an optical centrifuge, allowing for the study of molecular dynam…

physics.chem-ph2025

An optical centrifuge with zero rotational acceleration

K. Wang, A. Hardikar, A. A. Milner +1

An optical centrifuge is a laser pulse which enables controlled rotational excitation of molecules. Centrifuged molecules rotating with well-defined angular frequencies are ideal c…

quant-ph2023

Coherent control of molecular rotation in superfluid helium

Alexander A. Milner, Ian MacPhail-Bartley, Katarina Preocanin +3

We experimentally demonstrate control of molecular rotation in bulk superfluid . Metastable helium dimers, , are rotationally excited by a periodic…

physics.chem-ph2017★ 13 cited

Probing molecular potentials with an optical centrifuge

A. A. Milner, A. Korobenko, J. W. Hepburn +1

We use an optical centrifuge to excite coherent rotational wave packets in NO, CS and OCS molecules with rotational quantum numbers reaching up to J=465, 690 and 1186, resp…

quant-ph2016★ 22 cited

Ultrafast magnetization of a dense molecular gas with an optical centrifuge

A. A. Milner, A. Korobenko, V. Milner

Strong laser-induced magnetization of oxygen gas at room temperature and atmospheric pressure is achieved experimentally on the sub-nanosecond time scale. The method is based on co…

physics.chem-ph2015★ 30 cited

Adiabatic field-free alignment of asymmetric top molecules with an optical centrifuge

A. Korobenko, V. Milner

We use an optical centrifuge to align asymmetric top molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the…

physics.optics2015★ 11 cited

Generating long sequences of high-intensity femtosecond pulses

Martin Bitter, Valery Milner

We present an approach to create pulse sequences extending beyond 150~picoseconds in duration, comprised of J femtosecond pulses. A quarter of the pulse train is produced by…

physics.optics2015★ 25 cited

From gyroscopic to thermal motion: a crossover in the dynamics of molecular superrotors

A. A. Milner, A. Korobenko, K. Rezaiezadeh +1

Localized heating of a gas by intense laser pulses leads to interesting acoustic, hydrodynamic and optical effects with numerous applications in science and technology, including c…

physics.chem-ph2015★ 12 cited

Sound emission from the gas of molecular superrotors

A. A. Milner, A. Korobenko, V. Milner

We use an optical centrifuge to deposit a controllable amount of rotational energy into dense molecular ensembles. Subsequent rotation-translation energy transfer, mediated by ther…

quant-ph2014★ 3 cited

Magneto-optical properties of paramagnetic superrotors

A. A. Milner, A. Korobenko, J. Floß +2

We study the dynamics of paramagnetic molecular superrotors in an external magnetic field. Optical centrifuge is used to create dense ensembles of oxygen molecules in ultra-high ro…

physics.optics2012★ 27 cited

Directional spinning of molecules with sequences of femtosecond pulses

C. Bloomquist, S. Zhdanovich, A. A. Milner +1

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecul…

quant-ph2012★ 61 cited

Quantum resonances in selective rotational excitation of molecules with a sequence of ultrashort laser pulses

S. Zhdanovich, C. Bloomquist, J. Floß +3

We investigate experimentally the effect of quantum resonance in the rotational excitation of the simplest quantum rotor - a diatomic molecule. By using the techniques of high-reso…

quant-ph2011★ 84 cited

Control of molecular rotation with a chiral train of ultrashort pulses

S. Zhdanovich, A. A. Milner, C. Bloomquist +4

Trains of ultrashort laser pulses separated by the time of rotational revival (typically, tens of picoseconds) have been exploited for creating ensembles of aligned molecules. In t…

physics.atom-ph2007★ 77 cited

Population transfer between two quantum states by piecewise chirping of femtosecond pulses: Theory and experiment

S. Zhdanovich, E. A. Shapiro, M. Shapiro +2

We propose and demonstrate the method of population transfer by piecewise adiabatic passage between two quantum states. Coherent excitation of a two-level system with a train of ul…