activity
20132026
most citedDouble core hole production in N2: Beating the Auger clock

180 citations · 187 across the 8 of their papers we have counts for

collaborators

8 papers

physics.optics2026

Roadmap on Attosecond Science

Rocio Borrego Varillas, Pierre Agostini, Fernando Ardana-Lamas +108

Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time…

physics.atom-ph2026

Coherent vibrational dynamics in molecular bond breaking: methyl radical umbrella mode probed by femtosecond x-ray spectroscopy

Christian A. Schröder, John H. Hack, Joshua L. Edwards +6

We report on the observation of coherent molecular vibrations launched by the breaking of a molecular bond. The methyl radical, which is produced by photodissoci…

physics.optics2025★ 1 cited

All-optical logic gates for extreme ultraviolet switching via attosecond four-wave mixing

Patrick Rupprecht, Daniel M. Neumark, Stephen R. Leone

All-optical logic-gate-based switching is a prerequisite for photonic computing. This article introduces a logic-gate protocol for noncollinear four-wave mixing (FWM) of one attose…

physics.atom-ph2025

Probing autoionization decay lifetimes of the core-excited states in xenon using attosecond noncollinear four-wave-mixing spectroscopy

Nicolette G. Puskar, Patrick Rupprecht, Jan Dvořák +6

The decay of core-excited states is a sensitive probe of autoionization dynamics and correlation effects in many-electron systems, occurring on the fastest timescales. Xenon, with…

physics.chem-ph2025

Tracing long-lived atomic coherences generated via molecular conical intersections

Patrick Rupprecht, Francesco Montorsi, Lei Xu +7

Accessing coherences is key to fully understand and control ultrafast dynamics of complex quantum systems like molecules. Most photochemical processes are mediated by conical inter…

physics.atom-ph2024

Extracting doubly-excited state lifetimes in helium directly in the time domain with attosecond noncollinear four-wave-mixing spectroscopy

Patrick Rupprecht, Nicolette G. Puskar, Daniel M. Neumark +1

The helium atom, with one nucleus and two electrons, is a prototypical system to study quantum many-body dynamics. Doubly-excited states, or quantum states in which both electrons…

physics.chem-ph2024★ 6 cited

Measurement of Coherent Vibrational Dynamics with X-ray Transient Absorption Spectroscopy Simultaneously at the Carbon K- and Chlorine L- Edges

Andrew D. Ross, Diptarka Hait, Valeriu Scutelnic +3

X-ray Transient Absorption Spectroscopy near the carbon K-edge (1s, 285 eV) and chlorine L edges (2p, 200 eV) is used to study the nuclear dynamics of CCl…

physics.acc-ph2013★ 180 cited

Double core hole production in N2: Beating the Auger clock

L. Fang, M. Hoener, O. Gessner +16

We investigate the creation of double K-shell holes in N2 molecules via sequential absorption of two photons on a timescale shorter than the core-hole lifetime by using intense x-r…