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Ergodicity breaking in rapidly rotating C60 fullerenes
Lee R. Liu, Dina Rosenberg, P. Bryan Changala +5
Ergodicity, the central tenet of statistical mechanics, requires that an isolated system will explore all of its available phase space permitted by energetic and symmetry constrain…
Collision-induced C_60 rovibrational relaxation probed by state-resolved nonlinear spectroscopy
Lee R. Liu, P. Bryan Changala, Marissa L. Weichman +6
Quantum state-resolved spectroscopy was recently achieved for C60 molecules when cooled by buffer gas collisions and probed with a midinfrared frequency comb. This rovibrational qu…
Direct Frequency Comb Measurement of OD + CO -> DOCO Kinetics
Bryce J. Bjork, Thinh Q. Bui, Oliver H. Heckl +9
The kinetics of the OH + CO reaction, fundamental to both atmospheric and combustion chemistry, are complex due to the formation of the HOCO intermediate. Despite extensive studies…
Quantum-State Controlled Chemical Reactions of Ultracold KRb Molecules
S. Ospelkaus, K. -K. Ni, D. Wang +7
How does a chemical reaction proceed at ultralow temperatures? Can simple quantum mechanical rules such as quantum statistics, single scattering partial waves, and quantum threshol…