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Beyond Panchromatic Absorption: Deciphering the Excited-State Maze from Light Absorption to Photocatalysis in Dye-Sensitized MOFs
Manuela L. Kim, Mauricio E. Calvo, Katsuya Teshima +2
Metal--organic frameworks (MOFs) are promising photocatalysts whose visible-light absorption can be extended through linker functionalization; however, a red-shifted absorption edg…
Tuning Optoelectronic Properties and Photoelectrochemical Performance of \b{eta}-TaON via Vanadium Doping
Mirabbos Hojamberdiev, Ronald Vargas, Lorean Madriz +7
The application of beta-TaON for solar-driven water splitting is hindered by limitations in phase purity, stoichiometry, crystallinity, visible-light absorption, carrier mobility,…
Mechanistic Origin of Charge Separation and Enhanced Photocatalytic Activity in D--A-Functionalized UiO-66-NH MOFs
Anastasiia Kultaeva, Volodymyr Vasylkovskyi, Andreas Sperlich +4
Donor--acceptor (D--A) functionalization of MOF linkers can enhance visible-light photocatalytic activity, yet the mechanisms responsible for these effects remain unclear. He…
Unveiling Linker-Born Electron Spin Centers in UiO-66-NH2 MOF
Timur Biktagirov, Eugenio Otal, Leopold Trost +6
Metal-organic frameworks (MOFs), with their high porosity and large internal surface area, provide versatile platforms for integrating spin centers with potential applications in c…