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7 papers

physics.optics2026

Triple-Resonance Spectroscopy Using a Cavity-Enhanced Frequency Comb Probe

Qinxue Nie, Vinicius Silva de Oliveira, Adrian Hjältén +3

Accurate experimentally verified models of molecular hot-band transitions are essential for interpreting high-temperature spectra in environments ranging from exoplanetary atmosphe…

physics.chem-ph2026

Measurement and assignment of 10 rotational energy levels in the 9510 to 9810 cm and 6590 to 6900 cm ranges of methane using optical frequency comb double-resonance spectroscopy

Yuan Cao, Adrian Hjältén, Vinicius Silva de Oliveira +4

The paper reports measurements and assignments of methane rotational transitions with J ≥ 10 using optical‑optical double‑resonance spectroscopy combined with a cavity‑enhanced fre…

physics.chem-ph2026

Rotational energy levels in the ground vibrational state of methane with kHz-level accuracy from comb-referenced double-resonance and Lamb-dip spectroscopies

Vinicius Silva de Oliveira, Isak Silander, Hiroyuki Sasada +4

Methane is a key spherical-top molecule, yet restrictive selection rules for one-photon transitions have prevented determination of its ground state (GS) energies with state-of-the…

physics.chem-ph2026

Optical frequency comb double-resonance spectroscopy of the 9030-9175 cm states of ethylene

Adrian Hjältén, Vinicius Silva de Oliveira, Yuan Cao +3

We use optical-optical double-resonance (OODR) spectroscopy to measure for the first time hot-band transitions of ethylene (CH) between states in the 3000 cm and…

physics.chem-ph2025

Measurement and assignment of E-symmetry states in the 6010-6110 cm and 8940-9150 cm ranges of methane using optical frequency comb double-resonance spectroscopy

Adrian Hjältén, Vinicius Silva de Oliveira, Michael Rey +3

We use sub-Doppler optical-optical double-resonance (OODR) spectroscopy with a 3.3 m single-frequency pump and a cavity-enhanced 1.65 m comb probe to measure 33 ladder-type…

physics.optics2025

Combined frequency comb and continuous wave cavity-enhanced optical-optical double-resonance spectrometer in the 1.7 m range

Vinicius Silva de Oliveira, Adrian Hjältén, Isak Silander +4

We present an optical-optical double-resonance (OODR) spectrometer based on a 3.3 m continuous wave pump and two cavity-enhanced probes: a frequency comb tunable in the 1.64 -…