paper

Significant suppression of weak ferromagnetism in (LaEu)CuO

arXiv:cond-mat/0212360 · doi:10.1103/PhysRevB.67.224401

Abstract

The magnetic structure of (LaEu)CuO has been studied by magnetization measurements of single crystals, which show antiferromagnetic long-range order below = 265 K and a structural phase transition at = 130 K. At , the Cu spin susceptibility exhibits almost the same behavior as that of LaCuO in the low-temperature orthorhombic phase, which indicates the existence of finite spin canting out of the CuO plane. At , the magnitude of the weak-ferromagnetic moment induced by the spin canting is suppressed approximately by 70{%}. This significant suppression of the weak-ferromagnetic moment is carefully compared with the theoretical analysis of weak ferromagnetism by Stein {\it et al.} (Phys. Rev. B {\bf 53}, 775 (1996)), in which the magnitude of weak-ferromagnetic moments strongly depend on the crystallographic symmetry. Based on such comparison, below (LaEu)CuO is in the low-temperature less-orthorhombic phase with a space group of . We also discuss the possible magnetic structure of the pure low-temperature tetragonal phase with space group , which is relevant for rare-earth and alkaline-earth ions co-doped LaCuO.

16 pages including 5 figures, submitted to Phys. Rev. B. Fig. 4 is newly added

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