Zone-boundary excitations in coupled Haldane spin chain compounds PbNi2V2O8 and SrNi2V2O8

Abstract

Magnetic excitations in the quasi-one-dimensional quantum antiferromagnets PbNi2V2O8 and SrNi2V2O8 are measured all the way up to the zone boundary energy using inelastic neutron scattering from powder samples. An estimate for next-nearest-neighbor in-chain interactions is obtained. The role played by these interactions in spin-vacancy induced magnetic ordering in PbNi2V2O8 is discussed.

submitted to Phys. Rev. B

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