Confinement, deconfinement, and bound states in the spin-$1$ and spin-$3/2$ generalizations of the Majumdar--Ghosh chain

Abstract

We investigate the nature of low-energy excitations in a spin chain with antiferrmomagnetic nearest-neighbor $J_1$, next-nearest-neighbor $J_2$, and three-site $J_3$ interactions using the time-dependent density matrix renormalization group and the single mode approximation techniques. In the absence of the $J_2$ interaction, we identify clear distinctions in the spectral functions in the fully dimerized phase across the exactly dimerized line for different magnitudes of the spins. In contrast to the spin-$1/2$ chain, where the spinon continuum dominates the spectral functions, the magnon modes are prominent in the spectral functions of the spin-$1$ and spin-$3/2$ chains. Through single mode approximation and valence bond solid approaches, we disentangle magnon and spinon contributions to the spectral functions. After including the $J_2$ interactions, for the spin-$1$ chain we trace the evolution of the dynamical structure factor along the phase transition line between the Haldane phase and the fully dimerized phase. We find that the excitation spectrum is a continuum along this line and the spectral gap closes as the order of the transition changes from first order to second order. Along the line of first-order transitions, the spinon-like domain walls are deconfined, and the model exhibits their confinement into discrete bound states away from the transition line. A similar phenomenon occurs in the spin-$3/2$ chain across the phase transition between partially dimerized to fully dimerized phases, revealing a universal spinon confinement phenomenon across first-order phase transitions. This study presents the dynamical structure factor corresponding to the ground state phase diagram and establishes a unified quasiparticle framework for understanding the fundamental nature of excitations across distinct quantum phases in frustrated $J_1$-$J_2$-$J_3$ Heisenberg spin chains.

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