Purcell-enhanced spin-phonon coupling with a single color center

Abstract

The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely used in quantum computing and communication to channel photons emitted by atoms into well-defined modes and control atom-photon interactions. For solid-state artificial atoms, such as color-centers, the host lattice introduces an acoustic environment, allowing excited atoms to relax by emitting phonons. Here we observe the acoustic Purcell effect by constructing a specially engineered, microwave-frequency nanomechanical resonator around a color-center spin qubit in diamond. Using a co-localized optical mode of the structure that strongly couples to the color-center's excited state, we perform single-photon-level laser spectroscopy at milliKelvin temperatures and observe ten-fold faster spin relaxation when the spin qubit is tuned into resonance with a 12 GHz acoustic mode. Additionally, we use the color-center as an atomic-scale probe to measure the broadband phonon spectrum of the nanostructure up to a frequency of 28 GHz. Our work establishes a new regime of control for quantum defects in solids and paves the way for interconnects between atomic-scale quantum memories and qubits encoded in acoustic and superconducting devices.

39 pages, 20 figures

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