Crystallization of the transdimensional electron liquid
arXiv:2503.05165 · doi:10.1021/acs.nanolett.5c03894
Abstract
Wigner crystallization of free electrons at room temperature is explored for a new class of metallic ultrathin (transdimensional) materials whose properties can be controlled by their thickness. Our calculations of the critical electron density, temperature and the melting curve show that by reducing the material thickness one can Wigner-crystallize free electrons at room temperature to get them pinned onto a two-dimensional triangular lattice of a supersolid inside of the crystalline material. Such a solid melts and freezes reversibly with increase and decrease of electron doping or temperature, whereby its resistivity behaves opposite to the free electron gas model predictions.
Main text and supplementary information; total of 14 pages and 7 figures
References in corpus (30)
- A Tunable Kondo Effect in Quantum Dots
- Optical detection of Mott and generalized Wigner crystal states in WSe2/WS2 moiré superlattices
- Dielectric screening in two-dimensional insulators: Implications for excitonic and impurity states in graphane
- Abundance of correlated insulating states at fractional fillings of WSe/WS moiré superlattices
- High-temperature superfluidity with indirect excitons in van der Waals heterostructures
- Correlated Insulating States at Fractional Fillings of the WS2/WSe2 Moiré Lattice
- Tunable plasmons in ultrathin metal films
- Strongly correlated excitonic insulator in atomic double layers
- Signatures of bilayer Wigner crystals in a transition metal dichalcogenide heterostructure
- Observation of Wigner crystal of electrons in a monolayer semiconductor
- Stripe phases in WSe2/WS2 moiré superlattices
- Wigner crystallization and metal-insulator transition of two-dimensional holes in GaAs/AlGaAs at B=0
- Tunable plasmons in atomically thin gold nanodisks
- Imaging the Wigner Crystal of Electrons in One Dimension
- Direct observation of a magnetic field-induced Wigner crystal
- Chiral excitonic order from twofold van Hove singularities in kagome metals
- Sharp Tunneling Resonance from the Vibrations of an Electronic Wigner Crystal
- Roadmap for Photonics with 2D Materials
- Wigner supersolid of excitons in electron-hole bilayers
- Skyrmion solids in monolayer graphene
- Universal features of the optical properties of ultrathin plasmonic films
- Roadmap on Nonlocality in Photonic Materials and Metamaterials
- Transdimensional epsilon-near-zero modes in planar plasmonic nanostructures
- Optical Response of Finite-Thickness Ultrathin Plasmonic Films
- Strong-coupling phases of trions and excitons in electron-hole bilayers at commensurate densities
- Far- and Near-Field Heat Transfer in Transdimensional Plasmonic Film Systems
- Kondo effect in electrostatically defined ZnO quantum dots
- Controlling Single-Photon Emission with Ultrathin Transdimensional Plasmonic Films
- Magnetic-Field-Induced Wigner Crystallization of Charged Interlayer Excitons in van der Waals Heterostructures
- Goos-Hänchen effect singularities in transdimensional plasmonic films