Spin excitations in bilayer La${}_3$Ni${}_2$O${}_7$ superconductors with the interlayer pairing

Abstract

Prompted by the recent discovery of high-temperature superconductivity in La${}_3$Ni${}_2$O${}_7$ under pressure, this study delves into a theoretical investigation of spin excitations within this intriguing material. Through self-consistent mean-field calculations, we propose that superconductivity in this compound is primarily driven by interlayer pairing mechanisms. This interlayer pairing results in an effective $s_{\pm }$ pairing gap, with the sign of the pairing gap varying across different Fermi pockets. In the superconducting state, our analysis reveals a striking absence of a spin resonance mode. Moreover, we reveal a spectrum of energy-dependent incommensurate spin excitations. The observed incommensurate structures are elegantly explained by the nesting effect of energy contours, providing a coherent and comprehensive account of experimental observations. The implications of these spin excitations in La${}_3$Ni${}_2$O${}_7$ are profound, offering critical insights into the superconducting mechanism at play. Our results not only contribute to the understanding of this novel superconductor but also pave the way for further research into the interplay between spin dynamics and unconventional superconductivity in layered materials.

12 pages, 10 figures

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• Decomposition of multilayer superconductivity with interlayer pairing
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Cited by in corpus (6)

• Effective perpendicular electric field as a probe for interlayer pairing in ambient-pressure superconducting La${}_{2.85}$Pr${}_{0.15}$Ni${}_2$O${}_7$ thin films
• General trends of electronic structures, superconducting pairing, and magnetic correlations in the Ruddlesden-Popper nickelate $m$-layered superconductors La${}_{m+1}$Ni${}_m$O${}_{3m+1}$
• Robust $s_{\pm }$-wave pairing in a bilayer two-orbital model of pressurized La${}_3$Ni${}_2$O${}_7$ without the $\gamma$ Fermi surface
• Compressive Strain Turns $s^{\pm }$ into $d$-Wave Pairing in One-unit-cell La${}_3$Ni${}_2$O${}_7$ Thin Film Via Substrate-Induced Hole Doping
• Probing Sign-Changing Order Parameters via Impurity States in unconventional superconductors: Implications for La${}_3$Ni${}_2$O${}_7$ Superconductors with interlayer pairing
• Layer-Resolved Impurity States Reveal Competing Pairing Mechanisms in Trilayer Nickelate Superconductor La${}_4$Ni${}_3$O${}_{10}$