Doping evolution of the normal state magnetic excitations in pressurized La3Ni2O7

Abstract

The doping evolution behaviors of the normal state magnetic excitations (MEs) of the nickelate La3Ni2O7 are theoretically studied in this paper. For a filling of n = 3.0 which corresponds roughly to the material which realizes the superconductivity of about 80 K under moderately high pressures above 14 GPa, the MEs exhibit a square-like pattern centered at (0,0) which originates from the intrapocket particle-hole scatterings. Furthermore, it was found that the MEs show very strong modulations on the interlayer momentum qz. With the increasing of qz, the patterns of the MEs change dramatically. In the large qz regime, they turn to be ruled by the interpocket excitation modes with significantly larger intensity which may play a vital role in the superconducting pairing. This hidden feature of the MEs was not revealed by previous studies. The established features of the MEs are found to be very robust against doping. They persist in the wide hole- or electron-doping regime around n = 3.0. However, in the heavily electron-doped regime, a Lifshitz transition will occur. Consequently, the behaviors of the MEs change qualitatively across this transition. With the absence of the hole pocket, we predict that a strong tendency toward the spin-density-wave (SDW) order will develop due to the perfect nesting between the electron and the hole pockets at n = 4.0. Thus, we have investigated the normal state behaviors of the MEs and their doping evolutions which may shed light on the mechanism of superconductivity in pressurized La3Ni2O7.

9 pages, 9 figures

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Cited by in corpus (5)

• Impact of Pressure and Apical Oxygen Vacancies on Superconductivity in La${}_3$Ni${}_2$O${}_7$
• Strong-coupling study of the pairing mechanism in pressurized La${}_3$Ni${}_2$O${}_7$
• Intertwined charge and spin instability of La${}_3$Ni${}_2$O${}_7$
• Unified mechanism of charge-density-wave and high-$T_c$ superconductivity protected from oxygen vacancies in bilayer nickelates
• Incommensurate spin fluctuations and competing pairing symmetries in La${}_3$Ni${}_2$O${}_7$