Finite-Temperature Hole-Magnon Dynamics in an Antiferromagnet
arXiv:2401.11184 · doi:10.1021/acs.jpclett.3c03298
Abstract
Employing the numerically accurate multiple Davydov Ansatz in combination with the thermo-field dynamics approach, we delve into interplay of the finite-temperature dynamics of holes and magnons in an antiferromagnet, which allows for scrutinizing previous predictions from self-consistent Born approximation while offering, for the first time, accurate finite-temperature computation of detailed magnon dynamics as a response and a facilitator to the hole motion. The study also uncovers pronounced temperature dependence of the magnon and hole populations, pointing to the feasibility of potential thermal manipulation and control of hole dynamics. Our methodology can be applied not only to the calculation of steady-state angular-resolved photoemission spectra, but also to the simulation of femtosecond terahertz pump-probe and other nonlinear signals for the characterization of antiferromagnetic materials.
28 pages, 5 figures
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