Probing the Anomalous Hall Transport and Magnetic Reversal of Chiral-Lattice Antiferromagnet Co${}_{1/3}$NbS${}_2$

Abstract

Antiferromagnets exhibiting giant anomalous Hall effect (AHE) and anomalous Nernst effect (ANE) have recently aroused broad interest, not only for their potential applications in future electronic devices, but also because of the rich physics arising from the Berry curvature near the Fermi level. $\mathrm{C}{\mathrm{o}}_{1/3}\mathrm{Nb}{\mathrm{S}}_2$, by intercalating $\mathrm{C}{\mathrm{o}}^{2+}$ ions between $\mathrm{Nb}{\mathrm{S}}_2$ layers, is a quasi-two-dimensional layered antiferromagnet with a chiral lattice. A large AHE has been observed in $\mathrm{C}{\mathrm{o}}_{1/3}\mathrm{Nb}{\mathrm{S}}_2$, but its origin is under debate. In this letter, we report the large AHE and ANE in exfoliated $\mathrm{C}{\mathrm{o}}_{1/3}\mathrm{Nb}{\mathrm{S}}_2$ flakes. By analyzing the thermoelectric data via the Mott relation, we determined that the observed large AHE and ANE primarily result from the intrinsic Berry curvature. We also observed the magnetic domains in $\mathrm{C}{\mathrm{o}}_{1/3}\mathrm{Nb}{\mathrm{S}}_2$ by reflective magnetic circular dichroism measurements. Combined with electrical transport measurements, we confirmed that the magnetic reversal in $\mathrm{C}{\mathrm{o}}_{1/3}\mathrm{Nb}{\mathrm{S}}_2$ is determined by domain wall motion, and the critical field ($H_c$) exhibits a memory effect of consecutive magnetic sweeps. Our work provides insight into the topological properties of $\mathrm{C}{\mathrm{o}}_{1/3}\mathrm{Nb}{\mathrm{S}}_2$ and paves the way to studying the spin configuration and magnetic domain dynamics in this fascinating antiferromagnet.

8 pages, 4 figures

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