Exceptional points treatment of cavity spectroscopies

Abstract

The infrared response of a system of two vibrational modes in a cavity is calculated by an effective non-Hermitian Hamiltonian derived by employing the nonequilibrium Green's functions (NEGF) formalism. Degeneracies of the Hamiltonian (exceptional points, EP) widely employed in theoretical analysis of optical cavity spectroscopies are used in an approximate treatment and compared with the full NEGF. Qualitative limitations of the EP treatment are explained by examining the approximations employed in the calculation.

This article may be downloaded for personal use only. Any other use requires prior permission of the author and AIP Publishing. This article appeared in J. Chem. Phys. 158, 154106 (2023) and may be found at https://doi.org/10.1063/5.0142022 Copyright (2023) Authors. This article is distributed under a Creative Commons Attribution (CC BY) License

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• Liouvillian exceptional points of an open driven two-level system
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• Nonlinear optical spectroscopy of open quantum systems