Magnetic phase diagram and possible Kitaev-like behavior of honeycomb-lattice antimonate Na3Co2SbO6

Abstract

Recent theoretical studies have suggested that Kitaev physics and such effects as formation of a mysterious spin-liquid state can be expected not only in RuCl3 and iridates, but also in conventional $3d$ transition metal compounds. Using DC and AC magnetometry, thermodynamic and ${}^{23}$Na nuclear magnetic resonance measurements (NMR) we studied such a candidate material Na3Co2SbO6. A full phase diagram of Na3Co2SbO6 in a wide range of magnetic fields and temperatures is presented. The results demonstrate transformation of the antiferromagnetic structure under the external magnetic field, gradual development of the saturation phase, as well as evidence of gapped behavior in certain parts of the phase diagram

References in corpus (19)

• Pseudospin exchange interactions in d^7 cobalt compounds: Possible realization of the Kitaev model
• Orbital effects in solids: basics, recent progress and opportunities
• Kitaev-Heisenberg Hamiltonian for High-Spin $d^7$ Mott Insulators
• Kitaev Spin Liquid in 3d Transition Metal Compounds
• Field-induced quantum spin disordered state in spin-1/2 honeycomb magnet Na2Co2TeO6
• Kitaev interactions in the Co honeycomb antiferromagnets Na${}_3$Co${}_2$SbO${}_6$ and Na${}_2$Co${}_2$TeO${}_6$
• Weak-field induced nonmagnetic state in a Co-based honeycomb
• Antiferromagnetic Kitaev interaction in $J_\rm{eff}=1/2$ cobalt honeycomb materials Na${}_3$Co${}_2$SbO${}_6$ and Na${}_2$Co${}_2$TeO${}_6$
• Magnetic order in single crystals of Na3Co2SbO6 with a honeycomb arrangement of 3d${}^7$ Co${}^{2+}$ ions
• Dominant Kitaev interactions in the honeycomb materials Na${}_3$Co${}_2$SbO${}_6$ and Na${}_2$Co${}_2$TeO${}_6$
• Identification of Magnetic Interactions and High-field Quantum Spin Liquid in $\alpha$-RuCl${}_3$
• XY magnetism, Kitaev exchange, and long-range frustration in the $J_{\mathrm{eff}}=1/2$ honeycomb cobaltates
• Magnetic Couplings in Edge-Sharing High-Spin $d^7$ Compounds
• Ab initio guided minimal model for the "Kitaev" material BaCo${}_2$(AsO${}_4$)${}_2$: Importance of direct hopping, third-neighbor exchange and quantum fluctuations
• Giant magnetic in-plane anisotropy and competing instabilities in Na3Co2SbO6
• Synthesis, structure and magnetic properties of honeycomb-layered Li3Co2SbO6 with new data on its sodium precursor, Na3Co2SbO6
• Field evolution of magnetic phases and spin dynamics in the honeycomb lattice magnet Na2Co2TeO6: 23Na NMR study
• Exact solutions of few-magnon problems in the spin-$S$ periodic XXZ chain
• {23}Na nuclear spin-lattice relaxation studies of Na2Ni2TeO6

Cited by in corpus (15)

• Comparative Raman Scattering Study of Crystal Field Excitations in Co-based Quantum Magnets
• Field-induced phase transitions and quantum criticality in a honeycomb antiferromagnet Na3Co2SbO6
• Suppression of Antiferromagnetic Order by Strain in Honeycomb Cobaltate: Implication for Quantum Spin Liquid
• Persistent spin dynamics in magnetically ordered honeycomb cobalt oxides
• Advances in honeycomb layered oxides: Part I -- Syntheses and Characterisations of Pnictogen- and Chalcogen-Based Honeycomb Layered Oxides
• BaCo${}_2$(AsO${}_4$)${}_2$: Strong Kitaev, After All
• Probing critical spin fluctuations with a composite magnetoelectric method: A case study on a Kitaev spin liquid candidate Na${}_3$Co${}_2$SbO${}_6$
• Cobalt-Based Pyroxenes: A New Playground for Kitaev Physics and Ising Model Realization
• Signatures of a gapless quantum spin liquid in the Kitaev material Na${}_3$Co${}_{2-x}$Zn${}_x$SbO${}_6$
• Field-induced magnetic phases in the Kitaev candidate Na${}_3$Co${}_2$SbO${}_6$
• Raman spectroscopy of Na${}_3$Co${}_2$SbO${}_6$
• Coexistence of static and dynamic local magnetic fields in an S = 3/2 honeycomb lattice antiferromagnet Co2Te3O8
• Spin disorder state induced by Mg${}^{2+}$ doping in a Kitaev material Na${}_3$Co${}_2$SbO${}_6$
• Crystalline water intercalation into the Kitaev honeycomb cobaltate Na${}_2$Co${}_2$TeO${}_6$
• Kitaev interaction and possible spin liquid state in CoI2 and Co2/3Mg1/3I2