Mott-moiré excitons

Abstract

We develop a systematic theory for excitons subject to Fermi-Hubbard physics in moiré twisted transition metal dichalcogenides (TMDs). Specifically, we consider excitons in moiré systems for which the valence band is in the Mott-insulating regime. These "Mott-moiré excitons", which are achievable in twisted TMD heterobilayers, are bound states of a magnetic polaron in the valence band and a free electron in the conduction band. We find significantly narrower exciton bandwidths in the presence of Hubbard physics, serving as a potential experimental signature of strong correlations. We also demonstrate the high tunability of Mott-moiré excitons through the dependence of their binding energies, diameters, and bandwidths on the moiré period. Our work provides guidelines for future exploration of strongly correlated excitons in twisted TMD heterobilayers.

References in corpus (35)

• Resonantly hybridised excitons in moiré superlattices in van der Waals heterostructures
• Abundance of correlated insulating states at fractional fillings of WSe${}_2$/WS${}_2$ moiré superlattices
• Moiré heterostructures as a condensed matter quantum simulator
• Exciton band structure of monolayer MoS2
• Continuous Mott transition in semiconductor moiré superlattices
• Theory of optical absorption by interlayer excitons in transition metal dichalcogenide heterobilayers
• Many-Body Theory of Trion Absorption Features in Two-Dimensional Semiconductors
• Stripe phases in WSe2/WS2 moiré superlattices
• Imaging moiré flat bands in 3D reconstructed WSe2/WS2 superlattices
• Strongly-Correlated Electron-Photon Systems
• Band topology, Hubbard model, Heisenberg model, and Dzyaloshinskii-Moriya interaction in twisted bilayer WSe${}_2$
• Realization of an atomically thin mirror using monolayer MoSe2
• Effective spin model for the spin-liquid phase of the Hubbard model on the triangular lattice
• Tunable bilayer Hubbard model physics in twisted WSe2
• Quantum Phase Diagram of a Moiré-Hubbard Model
• Hartree-Fock study of the moiré Hubbard model for twisted bilayer transition metal dichalcogenides
• Correlated interlayer exciton insulator in double layers of monolayer WSe2 and moiré WS2/WSe2
• Electronic structures, charge transfer and charge orders in twisted transition metal dichalcogenide bilayers
• Coupling a mobile hole to an antiferromagnetic spin background: Transient dynamics of a magnetic polaron
• Charge Transfer Excitations, Pair Density Waves, and Superconductivity in Moiré Materials
• Microscopic spinon-chargon theory of magnetic polarons in the t-J model
• Confinement-Deconfinement Transition as an Indication of Spin-Liquid-Type Behavior in Na${}_2$IrO${}_3$
• Competing magnetic states in transition metal dichalcogenide moiré materials
• Hole Spectral Function of a Chiral Spin Liquid in the Triangular Lattice Hubbard Model
• Spontaneous valley polarization of interacting carriers in a monolayer semiconductor
• Moiré-induced optical non-linearities: Single and multi-photon resonances
• Spin-Mediated Mott Excitons
• The strong modulation limit of excitons and trions in moiré materials
• Proposal for asymmetric photoemission and tunneling spectroscopies in quantum simulators of the triangular-lattice Fermi-Hubbard model
• Doping a Mott insulator with excitons in moiré bilayer: fractional superfluid, neutral Fermi surface and Mott transition
• Composite boson many-body theory for Frenkel excitons
• Superconductivity in Engineered Two-Dimensional Electron Gases
• Optical signatures of periodic magnetization: the moiré Zeeman effect
• Antiferromagnetic, metal-insulator, and superconducting phase transitions in underdoped cuprates: Slave-fermion t-J model in the hopping expansion
• Signature of electromagnetic quantum fluctuations in exciton physics

Cited by in corpus (10)

• Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moiré ${\mathrm{WS}}_2$/${\mathrm{WSe}}_2$ heterobilayer
• Polaron spectroscopy of interacting Fermi systems: insights from exact diagonalization
• Non-bosonic moiré excitons
• Collective optical properties of moiré excitons
• Exciton and light induced ferromagnetism from doping a moiré Mott insulator
• Exciton interacting with a moiré lattice: Polarons, strings, and optical probing of spin correlations
• Electrically tunable and enhanced nonlinearity of moiré exciton-polaritons in transition metal dichalcogenide bilayers
• Purely electronic model for exciton-polaron formation in moiré heterostructures
• Correlated phases of moat-band excitons in two dimensions
• Probing spatially resolved spin density correlations with trapped excitons