Prototypical many-body signatures in transport properties of semiconductors
arXiv:2112.07604 · doi:10.1103/PhysRevB.105.085139
Abstract
We devise a methodology for charge, heat, and entropy transport driven by carriers with finite lifetimes. Combining numerical simulations with analytical expressions for low temperatures, we establish a comprehensive and thermodynamically consistent phenomenology for transport properties in semiconductors. We demonstrate that the scattering rate (inverse lifetime) is a relevant energy scale: It causes the emergence of several characteristic features in each transport observable. The theory is capable to reproduce -- with only a minimal input electronic structure -- the full temperature profiles measured in correlated narrow-gap semiconductors. In particular, we account for the previously elusive low- saturation of the resistivity and the Hall coefficient, as well as the (linear) vanishing of the Seebeck and Nernst coefficient in systems, such as FeSb, FeAs, RuSb and FeGa.
31 pages, 13 figures
References in corpus (19)
- BoltzTraP. A code for calculating band-structure dependent quantities
- Perturbo: a software package for ab initio electron-phonon interactions, charge transport and ultrafast dynamics
- On the thermoelectricity of correlated electrons in the zero-temperature limit
- The Nernst effect and the boundaries of the Fermi liquid picture
- Large Seebeck Effect by Charge-Mobility Engineering
- Optical properties of correlated materials -- Generalized Peierls approach and its application to VO2
- Thermopower of correlated semiconductors : application to FeAs2 and FeSb2
- Huge Thermoelectric Power Factor: FeSb2 versus FeAs2 and RuSb2
- Phonon-drag effect in FeGa3
- Transport, Thermal, and Magnetic Properties of the Narrow-Gap Semiconductor CrSb2
- Unified picture for the colossal thermopower compound FeSb
- Anisotropy in magnetic and transport properties of Fe1-xCoxSb2
- Longitudinal and anomalous Hall conductivity of a general two-band model
- Electronic correlations in FeGa and the effect of hole doping on its magnetic properties
- Vacancy defect control of colossal thermopower in FeSb2
- Resistivity saturation in Kondo insulators
- Diagrammatic study of optical excitations in correlated systems
- The role of electron-electron collisions for charge and heat transport at intermediate temperatures
- Resistivity Exponents in 3D-Dirac Semimetals From Electron-Electron Interaction