Prototypical many-body signatures in transport properties of semiconductors
arXiv:2112.07604 · doi:10.1103/PhysRevB.105.085139
Abstract
We devise a methodology for charge, heat, and entropy transport driven by carriers with finite lifetimes. Combining numerical simulations with analytical expressions for low temperatures, we establish a comprehensive and thermodynamically consistent phenomenology for transport properties in semiconductors. We demonstrate that the scattering rate (inverse lifetime) is a relevant energy scale: It causes the emergence of several characteristic features in each transport observable. The theory is capable to reproduce -- with only a minimal input electronic structure -- the full temperature profiles measured in correlated narrow-gap semiconductors. In particular, we account for the previously elusive low- saturation of the resistivity and the Hall coefficient, as well as the (linear) vanishing of the Seebeck and Nernst coefficient in systems, such as FeSb, FeAs, RuSb and FeGa.
arXiv comment31 pages, 13 figures
References in corpus (47)
- BoltzTraP. A code for calculating band-structure dependent quantities
- BoltzTraP2, a program for interpolating band structures and calculating semi-classical transport coefficients
- EPW: Electron-phonon coupling, transport and superconducting properties using maximally localized Wannier functions
- First-principles calculations of charge carrier mobility and conductivity in bulk semiconductors and two-dimensional materials
- BoltzWann: A code for the evaluation of thermoelectric and electronic transport properties with a maximally-localized Wannier functions basis
- The onset of the vortex-like Nernst signal above Tc in La_{2-x}Sr_xCuO_4 and Bi_2Sr_{2-y}La_yCuO_6
- Perturbo: a software package for ab initio electron-phonon interactions, charge transport and ultrafast dynamics
- On the thermoelectricity of correlated electrons in the zero-temperature limit
- Nernst effect in metals and superconductors: a review of concepts and experiments
- The Nernst effect and the boundaries of the Fermi liquid picture
- Large Seebeck Effect by Charge-Mobility Engineering
- Kondo Insulator description of spin state transition in FeSb2
- Ab initio optimization of phonon drag effect for lower-temperature thermoelectric energy conversion
- Signatures of electronic correlations in iron silicide
- Optical properties of correlated materials -- Generalized Peierls approach and its application to VO2
- Wiedemann-Franz law and Fermi liquids
- Thermal Transport for Many Body Tight-Binding Models
- Thermopower of correlated semiconductors : application to FeAs2 and FeSb2
- Conductivity in the square lattice Hubbard model at high temperatures: importance of vertex corrections
- Thermoelectricity in correlated narrow-gap semiconductors
- Huge Thermoelectric Power Factor: FeSb2 versus FeAs2 and RuSb2
- Thermoelectric properties of Co, Ir, and Os-Doped FeSi Alloys: Evidence for Strong Electron-Phonon Coupling
- Optical investigation of the metal-insulator transition in
- Nernst effect, quasiparticles, and d-density waves in cuprates
- Generic optical excitations of correlated systems: -tons
- Phonon-drag effect in FeGa3
- General Formula for the Thermoelectric Transport Phenomena based on the Fermi Liquid Theory: Thermopower, Nernst Coefficient, and Thermal Conductivity
- Transport, Thermal, and Magnetic Properties of the Narrow-Gap Semiconductor CrSb2
- Unified picture for the colossal thermopower compound FeSb
- Anisotropy in magnetic and transport properties of Fe1-xCoxSb2
- Longitudinal and anomalous Hall conductivity of a general two-band model
- Electronic correlations in FeGa and the effect of hole doping on its magnetic properties
- Highly Dispersive Electron Relaxation and Colossal Thermoelectricity in the Correlated Semiconductor FeSb
- Fate of a topological invariant for correlated lattice electrons at finite temperature
- Metallic surface states in a correlated d-electron topological Kondo insulator candidate FeSb2
- Vacancy defect control of colossal thermopower in FeSb2
- Unusual electronic and vibrational properties in the colossal thermopower material FeSb
- Anisotropic Correlated Electronic Structure of Colossal Thermopower Marcasite FeSb
- Resistivity saturation in Kondo insulators
- Hall and Faraday effects in interacting multi-band systems with arbitrary band topology and spin-orbit coupling
- Diagrammatic study of optical excitations in correlated systems
- Origin of the energy gap in the narrow-gap semiconductor FeSb2 revealed by high-pressure magnetotransport measurements
- The role of electron-electron collisions for charge and heat transport at intermediate temperatures
- Pressure-Driven Valence Increase and Metallization in Kondo Insulator CeBiPt
- Resistivity Exponents in 3D-Dirac Semimetals From Electron-Electron Interaction
- Composition induced metal-insulator quantum phase transition in the Heusler type Fe2VAl
- Electronic structure and thermoelectric properties of CoAsSb with post-DFT approaches