Artificial heavy fermions in a van der Waals heterostructure

Abstract

Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. They have been used as a platform for investigating exotic behavior ranging from quantum criticality and non-Fermi liquid behavior to unconventional topological superconductivity. Heavy fermions arise from the exchange interaction between localized magnetic moments and conduction electrons that leads to the well-known Kondo effect. In a Kondo lattice, the interaction between the localized moments gives rise to a band with heavy effective mass. This intriguing phenomenology has so far only been realized in compounds containing rare-earth elements with 4f or 5f electrons. Here, we realize a designer van der Waals heterostructure where artificial heavy fermions emerge from the Kondo coupling between a lattice of localized magnetic moments and itinerant electrons in a 1T/1H-TaS${}_2$ heterostructure. We study the heterostructure using scanning tunneling microscopy (STM) and spectroscopy (STS) and show that depending on the stacking order of the monolayers, we can either reveal the localized magnetic moments and the associated Kondo effect, or the conduction electrons with a heavy-fermion hybridization gap. Our experiments realize an ultimately tuneable platform for future experiments probing enhanced many-body correlations, dimensional tuning of quantum criticality, and unconventional superconductivity in two-dimensional artificial heavy-fermion systems.

References in corpus (26)

• Van der Waals heterostructures
• 2D materials and van der Waals heterostructures
• Fermi-liquid instabilities at magnetic quantum phase transitions
• Quantum Criticality in Heavy Fermion Metals
• Characterization of collective ground states in single-layer NbSe2
• Moiré heterostructures as a condensed matter quantum simulator
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• Is 1T-TaS${}_2$ a 40 year old quantum spin liquid?
• Topological Kondo Insulators
• Nanoscale manipulation of the Mott insulating state coupled to charge order in 1T-TaS2
• Visualizing Exotic Orbital Texture in the Single-Layer Mott Insulator 1T-TaSe2
• Visualizing heavy fermions emerging in a quantum critical Kondo lattice
• Imaging Cooper Pairing of Heavy Fermions in CeCoIn5
• Visualizing Nodal Heavy Fermion Superconductivity in CeCoIn5
• Imaging spinon density modulations in a 2D quantum spin liquid
• Temperature and magnetic field dependence of a Kondo system in the weak coupling regime
• Extremely strong coupling superconductivity in artificial two-dimensional Kondo lattices
• Hybridization gap and Fano resonance in SmB${}_6$
• The low-temperature highly correlated quantum phase in the charge-density-wave 1T-TaS_2 compound
• Emulating heavy fermions in twisted trilayer graphene
• Roles of the Narrow Electronic Band near the Fermi Level in 1T-TaS${}_2$-Related Layered Materials
• Evolution of the Kondo lattice and non-Fermi liquid excitations in a heavy-fermion metal
• Competition of Spinon Fermi Surface and Heavy Fermi Liquids states from the Periodic Anderson to the Hubbard model
• Topological Superconductivity in Metal/Quantum-Spin-Ice Heterostructures
• Chiral superconductivity in the alternate stacking compound 4Hb-TaS${}_2$

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• Heterogeneous Ta-dichalcogenide bilayer: heavy fermions or doped Mott physics?
• Unidirectional Kondo scattering in layered NbS2
• Nematic Ising superconductivity with hidden magnetism in few-layer 6R-TaS2
• Kondo-lattice-mediated interactions in flat band systems
• Roadmap on Nanoscale Superconductivity for Quantum Technologies