Understanding Reentrance in Frustrated Magnets: the Case of the Er${}_2$Sn${}_2$O${}_7$ Pyrochlore

Abstract

Reentrance, the return of a system from an ordered phase to a previously encountered less-ordered one as a controlled parameter is continuously varied, is a recurring theme found in disparate physical systems, from condensed matter to black holes. While diverse in its many incarnations and generally unsuspected, the cause of reentrance at the microscopic level is often not investigated thoroughly. Here, through detailed characterization and theoretical modeling, we uncover the microscopic mechanism behind reentrance in the strongly frustrated pyrochlore antiferromagnet Er${}_2$Sn${}_2$O${}_7$. Taking advantage of the recent advance in rare earth stannate single crystal synthesis, we use heat capacity measurements to expose that Er${}_2$Sn${}_2$O${}_7$ exhibits multiple instances of reentrance in its magnetic field $B$ vs. temperature $T$ phase diagram for magnetic fields along three cubic high symmetry directions. Through classical Monte Carlo simulations, mean field theory and classical linear spin-wave expansions, we argue that the origins of the multiple occurrences of reentrance observed in Er${}_2$Sn${}_2$O${}_7$ are linked to soft modes. Depending on the field direction, these arise either from a direct $T=0$ competition between the field-evolved ground states, or from a field-induced enhancement of the competition with a distinct zero-field antiferromagnetic phase. In both scenarios, the phase competition enhances thermal fluctuations which entropically stabilize a specific ordered phase. This results in an increased transition temperature for certain field values and thus the reentrant behavior. Our work represents a detailed examination into the mechanisms responsible for reentrance in a frustrated magnet and may serve as a template for the interpretation of reentrant phenomena in other physical systems.

arXiv commentMain text: 6 pages, 3 figures. Supplementary Material: 14 pages, 9 figures

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• Higher-Rank Spin Liquids and Spin Nematics from Competing Orders in Pyrochlore Magnets
• Traversing the pyrochlore stability diagram; microwave-assisted synthesis and discovery of mixed B-site Ln${}_2$InSbO${}_7$ family
• Quantum effects on pyrochlore higher-rank U(1) spin liquids: Pinch-line singularities, spin nematics, and connections to oxide materials
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