Materials preparation, single crystal growth, and the phase diagram of the cuprate high temperature superconductor La1.6-xNd0.4SrxCuO4
arXiv:2008.07573 · doi:10.1103/PhysRevMaterials.4.114801
Abstract
One branch of the La-214 family of cuprate superconductors, La1.6-xNd0.4SrxCuO4 (Nd-LSCO), has been of significant and sustained interest, in large part because it displays the full complexity of the phase diagram for canonical hole-doped, high Tc superconductivity, while also displaying relatively low superconducting critical temperatures. The low superconducting Tc's imply that experimentally accessible magnetic fields can suppress the superconductivity to zero temperature. In particular, this has enabled various transport and thermodynamic studies of the T = 0 ground state in Nd-LSCO, free of superconductivity, across the critical doping p* = 0.23 where the pseudogap phase ends. The strong dependence of its superconducting properties on its crystal symmetry has itself motivated careful studies of the Nd-LSCO structural phase diagram. This paper provides a systematic study and summary of the materials preparation and characterization of both single crystal and polycrystalline samples of Nd-LSCO. Single-phase polycrystalline samples with x spanning the range from 0.01 to 0.40 have been synthesized, and large single crystals of Nd-LSCO for select x across the region (0.07, 0.12, 0.17, 0.19, 0.225, 0.24, and 0.26) were grown by the optical floating zone method. Systematic neutron and X-ray diffraction studies on these samples were performed at both low and room temperatures, 10 K and 300 K, respectively. These studies allowed us to follow the various structural phase transitions and propose an updated structural phase diagram for Nd-LSCO. In particular, we found that the low-temperature tetragonal (LTT) phase ends at a critical doping pLTT = 0.255(5), clearly separated from p*.
31 pages, 15 figures
References in corpus (15)
- Mantid - Data Analysis and Visualization Package for Neutron Scattering and Experiments
- Change of carrier density at the pseudogap critical point of a cuprate superconductor
- Quantum critical point lying beneath the superconducting dome in iron-pnictides
- The remarkable underlying ground states of cuprate superconductors
- Thermodynamic signatures of quantum criticality in cuprates
- Giant thermal Hall conductivity from neutral excitations in the pseudogap phase of cuprates
- Pseudogap temperature of cuprate superconductors from the Nernst effect
- Fermi-surface transformation across the pseudogap critical point of the cuprate superconductor LaNdSrCuO
- The Persistence of High-Frequency Spin Fluctuations in Overdoped LaSrCuO (=0.22)
- Pseudogap phase of cuprate superconductors confined by Fermi surface topology
- Phase Diagram of BiSrCaCuO Revisited
- Electron scattering, charge order, and pseudogap physics in LaNdSrCuO: An angle resolved photoemission spectroscopy study
- Fermi surface transformation at the pseudogap critical point of a cuprate superconductor
- Spins, Stripes, and Superconductivity in Hole-Doped Cuprates
- Wiedemann-Franz law and abrupt change in conductivity across the pseudogap critical point of a cuprate superconductor
Cited by in corpus (7)
- Fermi surface transformation at the pseudogap critical point of a cuprate superconductor
- Vanishing nematic order beyond the pseudogap phase in overdoped cuprate superconductors
- Thermopower across the phase diagram of the cuprate LaNdSrCuO : signatures of the pseudogap and charge-density-wave phases
- Parallel Spin Stripes and Their Coexistance with Superconducting Ground States at Optimal and High Doping in LaNdSrCuO
- Superconductivity from charge order in cuprates
- Magnetic Field Tuning of Parallel Spin Stripe Order and Fluctuations near the Pseudogap Quantum Critical Point in LaNdSrCuO
- Dynamic Parallel Spin Stripes from the 1/8 anomaly to the End of Superconductivity in LaNdSrCuO