Multimode Organic Polariton Lasing
arXiv:2004.06679 · doi:10.1103/PhysRevLett.125.233603
Abstract
We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of non-lasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and non-lasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.
6 pages, 4 figures, plus supplemental material
References in corpus (23)
- Quantum fluids of light
- Room-temperature superfluidity in a polariton condensate
- Cavity-induced modifications of molecular structure in the strong coupling regime
- Plasmon-Exciton-Polariton Lasing
- Quantum theory of collective strong coupling of molecular vibrations with a microcavity mode
- An exciton-polariton laser based on biologically produced fluorescent protein
- Dark Vibronic Polaritons and the Spectroscopy of Organic Microcavities
- Suppressing and restoring the Dicke superradiance transition by dephasing and decay
- BCS-BEC crossover in a system of microcavity polaritons
- Tensor network simulation of non-Markovian dynamics in organic polaritons
- Excitonic spectral features in strongly-coupled organic polaritons
- Exact states and spectra of vibrationally dressed polaritons
- Polariton condensation with localised excitons and propagating photons
- Superradiant and Lasing States in Driven-Dissipative Dicke Models
- Microscopic Theory of Polariton Lasing via Vibronically Assisted Scattering
- Polariton condensation with saturable molecules dressed by vibrational modes
- Exciton-phonon scattering and photo-excitation dynamics in J-aggregate microcavities
- Sub-picosecond thermalization dynamics in condensation of strongly coupled lattice plasmons
- Cumulant expansion for the treatment of light-matter interactions in arbitrary material structures
- Room-Temperature Exciton-Polariton Condensation in a Tunable Zero-Dimensional Microcavity
- Tensor Network simulation of polaron-polaritons in organic microcavities
- Organic polariton lasing and the weak- to strong-coupling crossover
- Quantum emitter dipole-dipole interactions in nanoplasmonic systems
Cited by in corpus (27)
- Superabsorption in an organic microcavity: towards a quantum battery
- Theoretical Challenges in Polaritonic Chemistry
- Quantum Nanophotonics in Two-Dimensional Materials
- Uncovering Temperature-Dependent Exciton-Polariton Relaxation Mechanisms in Perovskites
- A theoretical perspective on molecular polaritonics
- Microscopic Theory of Multimode Polariton Dispersion in Multilayered Materials
- Efficient many-body non-Markovian dynamics of organic polaritons
- Generalization of the Tavis-Cummings model for multi-level anharmonic systems: insights on the second excitation manifold
- Determining the validity of cumulant expansions for central spin models
- Ultrafast collapse of molecular polaritons in photoswitch-nanoantennas at room temperature
- Exact analytical solution for density matrix of a non-equilibrium polariton Bose-Einstein condensate
- Wavelength-scale Optical Parametric Oscillators
- Polarization and phase textures in lattice plasmon condensates
- Mode switching dynamics in organic polariton lasing
- Self-hybridisation between interband transitions and Mie modes in dielectric nanoparticles
- Mean-field Mixed Quantum-Classical Approach for Many-Body Quantum Dynamics of Exciton-Polaritons
- Analytical framework for non-equilibrium phase transition to Bose--Einstein condensate
- Multiple Interacting Photonic Modes in Strongly Coupled Organic Microcavities
- Microscopic theory of nonlinear phase space filling in polaritonic lattices
- Thermalization rate of polaritons in strongly-coupled molecular systems
- Non-Markovian Dynamics of Open Quantum Systems via Auxiliary Particles with Exact Operator Constraint
- An analytic expression for the optical exciton transition rates in the polaron frame
- Raman-phonon-polariton condensation in a transversely pumped cavity
- Enhanced photoisomerization with hybrid metallodielectric cavities based on mode interference
- Non-Markovian effects in long-range polariton-mediated energy transfer
- Theory of dynamical superradiance in organic materials
- Collective Effects of Organic Molecules based on Holstein-Tavis-Cummings Model