Organic polariton lasing and the weak- to strong-coupling crossover
arXiv:1808.07683 · doi:10.1103/PhysRevLett.121.193601
Abstract
Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers.
arXiv comment6 pages, 4 figures, plus supplemental material
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Cited by in corpus (16)
- Molecular polaritons for controlling chemistry with quantum optics
- Polariton Localization and Dispersion Properties of Disordered Quantum Emitters in Multimode Microcavities
- Multimode Organic Polariton Lasing
- A theoretical perspective on molecular polaritonics
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- Nonlinear opto-vibronics in molecular systems
- Quantum heat transport in nonequilibrium anisotropic Dicke model