Spectroscopic Signatures of Electron-Phonon Coupling in Silicon-Vacancy Centers in Diamond
arXiv:2003.01118 · doi:10.1103/PhysRevMaterials.4.055202
Abstract
Vacancy centers in diamond have proven to be a viable solid-state platform for quantum coherent opto-electronic applications. Among the variety of vacancy centers, silicon-vacancy (SiV) centers have recently attracted much attention as an inversion-symmetric system that is less susceptible to electron-phonon interactions. Nevertheless, phonon-mediated processes still degrade the coherent properties of SiV centers, however characterizing their electron-phonon coupling is extremely challenging due to their weak spectroscopic signatures and remains an open experimental problem. In this paper we theoretically investigate signatures of electron-phonon coupling in simulated linear and nonlinear spectra of SiV centers. We demonstrate how even extremely weak electron-phonon interactions, such as in SiV centers, may be completely characterized via nonlinear spectroscopic techniques and even resolved between different fine-structure transitions.
References in corpus (20)
- Electron-phonon interactions from first principles
- Silicon-Vacancy Spin Qubit in Diamond: A Quantum Memory Exceeding 10 ms with Single-Shot State Readout
- The electronic structure of the silicon vacancy color center in diamond
- Quantum Nonlinear Optics with a Germanium-Vacancy Color Center in a Nanoscale Diamond Waveguide
- Multiple intrinsically identical single photon emitters in the solid-state
- All-optical initialization, readout, and coherent preparation of single silicon-vacancy spins in diamond
- Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond
- Electron-phonon processes of the silicon-vacancy centre in diamond
- Transform-limited photons from a coherent tin-vacancy spin in diamond
- Low temperature investigations of single silicon vacancy colour centres in diamond
- Controlling the coherence of a diamond spin qubit through strain engineering
- All-optical retrieval of the global phase for two-dimensional Fourier-transform spectroscopy
- Molecular vibrations-induced quantum beats in two-dimensional electronic spectroscopy
- Strongly inhomogeneous distribution of spectral properties of silicon-vacancy color centers in nanodiamonds
- Hybrid nanocavities for resonant enhancement of color center emission in diamond
- Vibrational Coupling Modifies Spectral Diffusion in Core-Shell Colloidal Quantum Dots
- Simultaneous Existence of Confined and Delocalized Vibrational Modes in Colloidal Quantum Dots
- Coherent control and wave mixing in an ensemble of silicon vacancy centers in diamond
- Effect of Dimensionality on the Optical Absorption Properties of CsPbI Perovskite Nanocrystals
- Microscopic modeling of the effect of phonons on the optical properties of solid-state emitters
Cited by in corpus (6)
- Towards Engineering Intrinsic Linewidths and Line-Broadening in Perovskite Nanoplatelets
- Spectral Broadening and Ultrafast Dynamics of a Nitrogen-Vacancy Center Ensemble in Diamond
- ODMR on Single TR12 Centers in Diamond
- Coherent Interactions Between Silicon-Vacancy Centers in Diamond
- Extracting Nonlinear Dynamical Response Functions from Time Evolution
- Measuring Exciton Fine-Structure in Perovskite Nanocrystal Ensembles