Magnetoelectric polarizability: A microscopic perspective

Abstract

We extend a field theoretic approach for the investigation of the electronic charge-current density response of crystalline systems to arbitrary applied electromagnetic fields. The approach leads to the introduction of microscopic polarization and magnetization fields, as well as free charge and current densities, the dynamics of which are described by a lattice gauge theory. The spatial averages of such quantities constitute the fields of macroscopic electrodynamics. We implement this formalism to study the orbital electronic response of a class of insulators to applied uniform dc electric and magnetic fields at zero temperature. To first-order in the applied fields, the free charge and current densities vanish; thus the response of the system is characterized by the first-order modifications to the microscopic polarization and magnetization fields. Associated with the dipole moment of the microscopic polarization (magnetization) field is a macroscopic polarization (magnetization), for which we extract various response tensors. We focus on the orbital magnetoelectric polarizability (OMP) tensor, and find the accepted expression as derived from the "modern theory of polarization and magnetization." Since our results are based on the spatial averages of microscopic fields, we can identify the distinct contributions to the OMP tensor from the perspective of this microscopic theory, and we establish the general framework in which extensions to finite frequency can be made.

24 pages

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• Magnetoelectric polarizability and optical activity: spin and frequency dependence
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• Electric polarization and magnetization in metals
• Symmetry, topology, and geometry: The many faces of the topological magnetoelectric effect
• Multipolar quantum electrodynamics of localized charge-current distributions: Spectral theory and renormalization
• Microscopic Theory of the Magnetic Susceptibility of Insulators
• Synthetic magnetoelectric response of lattice bosonic insulators
• Bulk versus surface: Nonuniversal partitioning of the topological magnetoelectric effect
• Chern insulators in two and three dimensions: A global perspective