Vibrational spectrum derived from the local mechanical response in disordered solids
arXiv:1907.06851 · doi:10.1039/D0SM00376J
Abstract
The low-frequency vibrations of glasses are markedly different from those of crystals. These vibrations have recently been categorized into two types: spatially extended vibrations, whose vibrational density of states (vDOS) follows a non-Debye quadratic law, and quasilocalized vibrations (QLVs), whose vDOS follows a quartic law. The former are explained by elasticity theory with quenched disorder and microscopic replica theory as being a consequence of elastic instability, but the origin of the latter is still debated. Here, we show that the latter can also be directly derived from elasticity theory with quenched disorder. We find another elastic instability that the theory encompasses but that has been overlooked so far, namely, the instability of the system against a local dipolar force. This instability gives rise to an additional contribution to the vDOS, and the spatial structure and energetics of the mode originating from this instability are consistent with those of the QLVs. Finally, we construct a model in which the additional contribution to the vDOS follows a quartic law.
arXiv comment9 pages, 1 figures
References in corpus (35)
- Amorphous Systems in Athermal, Quasistatic Shear
- Harmonic Vibrational Excitations in Disordered Solids and the "Boson Peak"
- Vibrational modes identify soft spots in a sheared disordered packing
- Continuum limit of the vibrational properties of amorphous solids
- Statistics and properties of low-frequency vibrational modes in structural glasses
- Continuum limit of amorphous elastic bodies (III): Three dimensional systems
- Marginal Stability in Structural, Spin and Electron Glasses
- Universal Spectrum of Normal Modes in Low-Temperature Glasses: an Exact Solution
- Low-frequency vibrational modes of stable glasses
- Statistical Physics of the Yielding Transition in Amorphous Solids
- Phase space geometry and slow dynamics
- Anharmonicity and quasi-localization of the excess low-frequency vibrations in jammed solids
- Anomalous properties of the acoustic excitations in glasses on the mesoscopic length-scale
- Universal non-phononic density of states in 2D, 3D and 4D glasses
- Scaling of phononic transport with connectivity in amorphous solids
- Geometric interpretation of pre-vitrification in hard sphere liquids
- The distribution of forces affects vibrational properties in hard sphere glasses
- Two-Level Systems and Boson Peak Remain Stable in 110-Million-Year-Old Amber Glass
- Universal non-Debye scaling in the density of states of amorphous solids
- Localised soft modes and the supercooled liquid's irreversible passage through its configuration space
- Spatial structure of quasi-localized vibrations in nearly jammed amorphous solids
- Phonon transport and vibrational excitations in amorphous solids
- Phonon gap and localization lengths in floppy materials
- A characteristic energy scale in glasses
- Nonlinear plastic modes in disordered solids
- Anomalous vibrational properties in the continuum limit of glasses
- Effect of instantaneous and continuous quenches on the density of vibrational modes in model glasses
- On Variational Arguments for Vibrational Modes near Jamming
- Spatial Distributions of Local Elastic Moduli Near the Jamming Transition
- Coherent-Potential approximation for diffusion and wave propagation in topologically disordered systems
- Theory for the density of interacting quasi-localised modes in amorphous solids
- Universal non-mean-field scaling in the density of state of amorphous solids
- Hydrodynamics of disordered marginally-stable matter
- Disorder-induced zero-energy spectral singularity for random matrices with correlations
- Anharmonic properties of vibrational excitations in amorphous solids
Cited by in corpus (21)
- Pinching a glass reveals key properties of its soft spots
- Low-energy quasilocalized excitations in structural glasses
- Low-frequency vibrational spectrum of mean-field disordered systems
- Mean-field model of interacting quasilocalized excitations in glasses
- A random matrix approach to the boson peak and Ioffe-Regel criterion in amorphous solids
- Universal non-Debye low-frequency vibrations in sheared amorphous solids
- Vibrational phenomena in glasses at low temperatures captured by field theory of disordered harmonic oscillators
- Low-Frequency Vibrational States in Ideal Glasses with Random Pinning
- Non-phononic density of states of two-dimensional glasses revealed by random pinning
- Bose-Einstein-Like condensation of deformed random matrix: A replica approach
- Random quench predicts universal properties of amorphous solids
- Spatial structure of unstable normal modes in a glass-forming liquid
- Properties of stable ensembles of Euclidean random matrices
- Understanding the scaling of boson peak through insensitivity of elastic heterogeneity to bending rigidity in polymer glasses
- Novel elastic instability of amorphous solids in finite spatial dimensions
- Intermittent rearrangements accompanying thermal fluctuations distinguish glasses from crystals
- Non-hyperuniform metastable states around a disordered hyperuniform state of densely packed spheres: stochastic density functional theory at strong coupling
- Instantaneous normal modes of glass-forming liquids during the athermal relaxation process of the steepest descent algorithm
- A self-consistent current response theory of jamming and vibrational modes in low-temperature amorphous solids
- Effective medium theory for viscoelasticity of soft jammed solids
- Unified study of viscoelasticity and sound damping in hard and soft amorphous solids