Unique defect structure and advantageous vortex pinning properties in superconducting CaKFe4As4

Abstract

The lossless current-carrying capacity of a superconductor is limited by its critical current density (Jc). A key to enhance Jc towards real-life applications is engineering defect structures to optimize the pinning landscape. For iron-based superconductors (IBSs) considered as candidate materials for high-field applications, high Jc values have been achieved by various techniques to introduce artificial pinning centres. Here we report extraordinary vortex pinning properties in CaKFe4As4 (CaK1144) arising from the inherent defect structure. Scanning transmission electron microscopy revealed the existence of nanoscale intergrowths of the CaFe2As2 phase, which is unique to CaK1144 formed as a line compound. The Jc properties in CaK1144 are found to be distinct from other IBSs characterized by a significant anisotropy with respect to the magnetic field orientation as well as a remarkable pinning mechanism significantly enhanced with increasing temperature. We propose a comprehensive explanation of the Jc properties based on the unique intergrowths acting as pinning centres.

15 pages, 5 figures, and Supplementary Information. One literature on the calculation of anisotropic Jc [S. Pyon, et al. Phys. Rev. B 99, 104506 (2019)] was added to the reference list

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• Expression with self-consistent magnetic units for calculation of critical current density using the Bean's Model
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• Synthesis of $c$-axis textured CaKFe${}_4$As${}_4$ superconducting bulk via spark plasma texturing technique
• Evolution of Critical Current Density in CaKFe${}_4$As${}_4$ with La-doping
• Low-field all-optical detection of superconductivity using NV nanodiamonds
• First-principles study of the electronic structure of CaKRu${}_4$P${}_4$