Circular holographic ionization-phase meter
arXiv:1904.04380 · doi:10.1103/PhysRevLett.123.133203
Abstract
We propose an attosecond XUV-pump IR-probe photoionization protocol that employs pairs of counter-rotating consecutive harmonics and angularly resolved photoelectron detection, thereby providing direct measurement of ionization phases. The present method, which we call circular holographic ionization-phase meter (CHIP), gives also access to the phase of photoemission amplitudes of even-parity continuum states from a single time-delay measurement, since the relative phase of one- and two-photon ionization pathways is imprinted in the photoemission anisotropy. The method is illustrated with \emph{ab initio} simulations of photoionization via autoionizing resonances in helium. The rapid phase excursion in the transition amplitude to both the dipole-allowed P and the dipole-forbidden D states are faithfully reproduced.
arXiv comment6 pages, 5 figures
References in corpus (16)
- Bright Coherent Ultrahigh Harmonics in the keV X-Ray Regime from Mid-Infrared Femtosecond Lasers
- Probing single-photon ionization on the attosecond time scale
- Generation of phase-matched circularly-polarized extreme ultraviolet high harmonics for magnetic circular dichroism spectroscopy
- Photoionization in the time and frequency domain
- Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron
- Nonsequential two-photon double ionization of helium
- Attosecond-resolved photoionization of chiral molecules
- Phase measurement of a Fano window resonance using tunable attosecond pulses
- Relaxation Dynamics in Photoexcited Chiral Molecules Studied by Time-Resolved Photoelectron Circular Dichroism: Toward Chiral Femtochemistry
- Two-photon finite-pulse model for resonant transitions in attosecond experiments
- Photoionization of helium by attosecond pulses: extraction of spectra from correlated wave functions
- Ionization branching ratio control with a resonance attosecond clock
- Probing electronic wavefunctions by all-optical attosecond interferometry
- Angular anisotropy of time delay in XUV/IR photoionization of H
- Polarization tagging of two-photon double ionization by elliptically polarized XUVs
- Application of the Complex Kohn Variational Method to Attosecond Spectroscopy
Cited by in corpus (9)
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- Dialogue on analytical and ab initio methods in attoscience
- Attosecond Ionization Time Delays in Strong-Field Physics
- Phase delays in above-threshold ionization
- Separation of Wigner and Continuum-continuum Delays by Mirror-symmetry-broken Attosecond Interferometry
- Angle-resolved time delays for shake-up ionization of helium
- Towards the complete phase profiling of attosecond wave packets
- Reconstruction of attosecond beating by interference of two-photon interband transitions in solids
- General properties of the RABBITT at parity mixing conditions