Observation of Bose-enhanced photoassociation products

Abstract

We produce ${}^{84}{\mathrm{Sr}}_2$ molecules using Bose-enhanced Raman photoassociation. We apply the stimulated Raman adiabatic passage (STIRAP) technique on a Bose-Einstein condensate (BEC) to produce more than $8\times 10^3$ ultracold molecules. This chemical reaction is only made possible because of the Bose enhancement of the optical transition dipole moment between the initial atomic state and an intermediate molecular state. We study the effect of Bose enhancement by measuring the transition Rabi frequency in a BEC and by comparing it with measurements for two atoms in sites of a Mott insulator. By breaking the dimers' bond and directly observing the separated atoms, we measure the molecular inelastic collision rate parameters. We discuss the possibility of applying Bose-enhanced STIRAP to convert a BEC of atoms into a BEC of molecules, and argue that the required efficiency for STIRAP is within experimental reach.

arXiv comment8 pages, 4 figures, 1 table

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Cited by in corpus (4)

• Ultracold ${}^{88}{\mathrm{Sr}}_2$ molecules in the absolute ground state
• Photoassociation of Ultracold NaLi
• High-intensity two-frequency photoassociation spectroscopy of a weakly bound molecular state: theory and experiment
• Highly Efficient Creation and Detection of Deeply-bound Molecules via Invariant-based Inverse Engineering with Feasible Modified Drivings