Induced Fission of Pu within a Real-Time Microscopic Framework
arXiv:1511.00738 · doi:10.1103/PhysRevLett.116.122504
Abstract
We describe the fissioning dynamics of Pu240 from a configuration in the proximity of the outer fission barrier to full scission and the formation of the fragments within an implementation of density functional theory extended to superfluid systems and real-time dynamics. The fission fragments emerge with properties similar to those determined experimentally, while the fission dynamics appears to be quite complex, with many excited shape and pairing modes. The evolution is found to be much slower than previously expected, and the ultimate role of the collective inertia is found to be negligible in this fully nonadiabatic treatment of nuclear dynamics, where all collective degrees of freedom (CDOF) are included (unlike adiabatic treatments with a small number of CDOF).
updated version in agreement with published paper, updated and new references, 7 pages, additional material at http://faculty.washington.edu/bulgac/Pu240/
References in corpus (24)
- Microscopic Theory of Nuclear Fission: A Review
- Brownian shape motion on five-dimensional potential-energy surfaces: Nuclear fission-fragment mass distributions
- Local Density Functional Theory for Superfluid Fermionic Systems: The Unitary Gas
- A Unitary Fermi Supersolid: The Larkin-Ovchinnikov Phase
- Total Prompt Energy Release in the Neutron-Induced Fission of 235-U, 238-U, and 239-Pu
- Particle number fluctuations and correlations in transfer reactions obtained using the Balian-Vénéroni variational principle
- Structure properties of Th and Fm fission fragments: mean field analysis with the Gogny force
- Fission dynamics within time-dependent Hartree-Fock: deformation-induced fission
- Pairing-induced speedup of nuclear spontaneous fission
- Microscopic modeling of mass and charge distributions in the spontaneous fission of 240Pu
- Dynamic versus static fission paths with realistic interactions
- Fission dynamics at low excitation energy. 2
- Final excitation energy of fission fragments
- Large Amplitude Dynamics of the Pairing Correlations in a Unitary Fermi Gas
- Fission dynamics within time-dependent Hartree-Fock: boost-induced fission
- Event-by-event study of prompt neutrons from 239Pu(n,f)
- Collective aspects deduced from time-dependent microscopic mean-field with pairing: application to the fission process
- Life Cycle of Superfluid Vortices and Quantum Turbulence in the Unitary Fermi Gas
- Relativistic Coulomb excitation within Time Dependent Superfluid Local Density Approximation
- Thermodynamics of nuclei in thermal contact
- Superfluid dynamics of 258Fm fission
- Nuclear Energy Density Functionals: What do we really know?
- Non-adiabatic dynamics of superfluid spin-orbit coupled degenerate Fermi gas
- Excitation of the dissipationless Higgs mode in a fermionic condensate
Cited by in corpus (131)
- Microscopic Theory of Nuclear Fission: A Review
- New states of matter with fine-tuned interactions: quantum droplets and dipolar supersolids
- Collisions of self-bound quantum droplets
- Review on the progress in nuclear fission
- Heavy-ions collisions and fission dynamics with the time-dependent Hartree-Fock theory and its extensions
- Superfluidity in nuclear systems and neutron stars
- Future of Nuclear Fission Theory
- r-Process Nucleosynthesis: Connecting Rare-Isotope Beam Facilities with the Cosmos
- Fission fragment charge and mass distributions in 239Pu(n,f) in the adiabatic nuclear energy density functional theory
- TDHF Theory and Its Extensions for the Multinucleon Transfer Reaction: a Mini Review
- Bayesian Evaluation of Incomplete Fission Yields
- Theory of Nuclear Fission
- Fission Dynamics of 240Pu from Saddle-to-Scission and Beyond
- Microscopic phase-space exploration modeling of Fm spontaneous fission
- Effect of shell structure on the fission of sub-lead nuclei
- Low-Energy Heavy-Ion Reactions and the Skyrme Effective Interaction
- Fission Fragment Decay Simulations with the CGMF Code
- Microscopic study of induced fission dynamics of Th with covariant energy density functionals
- Vortex pinning and dynamics in the neutron star crust
- Novel Role of Superfluidity in Low-Energy Nuclear Reactions
- Primary fission fragment mass yields across the chart of nuclides
- Nuclear Fission Dynamics: Past, Present, Needs, and Future
- Correlated Prompt Fission Data in Transport Simulations
- Fission fragments intrinsic spins and their correlations
- Angular Momentum of Fission Fragments from Microscopic Theory
- The time-dependent generator coordinate method in nuclear physics
- Time-dependent generator coordinate method study of mass-asymmetric fission of actinides
- Deformed shell effects in Ca+Bk quasifission fragments
- Multi-Nucleon Transfer in Central Collisions of U + U
- Formation and distribution of fragments in the spontaneous fission of 240Pu
- Measures of complexity and entanglement in fermionic many-body systems
- Microscopic analysis of induced nuclear fission dynamics
- Isotopic trends of quasifission and fusion-fission in the reactions Ca+Pu
- Microscopic predictions for production of neutron rich nuclei in the reaction
- Unitary evolution with fluctuations and dissipation
- Fission Dynamics of Compound Nuclei: Pairing versus Fluctuations
- Gauge angle dependence in TDHFB calculations of O + O head-on collisions with the Gogny interaction
- Entanglement entropy, single-particle occupation probabilities, and short-range correlations
- Microscopic Calculation of Fission Product Yields with Particle Number Projection
- Thermal fission rates with temperature dependent fission barriers
- Time-Dependent Density Functional Theory for Fermionic Superfluids: from Cold Atomic Gases, to Nuclei and Neutron Stars Crust
- Number of Particles in Fission Fragments
- Angular momentum of fission fragments
- Suppressed solitonic cascade in spin-imbalanced superfluid Fermi gas
- Coordinate-Space Solver for Superfluid Many-Fermion Systems with Shifted Conjugate Orthogonal Conjugate Gradient Method
- The influence of tensor force on the microscopic heavy-ion interaction potential
- Rotating quantum turbulence in the unitary Fermi gas
- Fission of Pu with symmetry-restored density functional theory
- Time-dependent generator coordinate method study of fission: dissipation effects
- First direct measurement of isotopic fission-fragment yields of U
- Isomeric fission yield ratios for odd-mass Cd and In isotopes using the Phase-Imaging Ion-Cyclotron-Resonance technique
- Dynamical effects in fusion with exotic nuclei
- Correlation studies of fission fragment neutron multiplicities
- Hauser-Feshbach fission fragment de-excitation with calculated macroscopic-microscopic mass yields
- Transfer probabilities for the reactions O+O in terms of multiple time-dependent Hartree-Fock-Bogoliubov trajectories
- Least action description of spontaneous fission in fermium and nobelium nuclei based on the Gogny energy density functional
- Dynamics of Fragmented Condensates and Macroscopic Entanglement
- Energy and pairing dependence of dissipation in real-time fission dynamics
- Microscopic description of pair transfer between two superfluid systems (II): a quantum mixing of Time-Dependent Hartree-Fock Bogolyubov trajectories
- Time-dependent covariant density functional theory in 3D lattice space: benchmark calculation for 16O + 16O reaction
- Time-dependent Hartree-Fock study of quasifission trajectories in reactions forming Og
- Scission configuration of U from yields and kinetic information of fission fragments
- Generalized time-dependent generator coordinate method for induced fission dynamics
- Fission dynamics, dissipation and clustering at finite temperature
- Neck Rupture and Scission Neutrons in Nuclear Fission
- Indirect methods in nuclear astrophysics with relativistic radioactive beams
- Improvements to the macroscopic-microscopic approach of nuclear fission
- The angular correlation between the fission fragment intrinsic spins
- Composite-particle decay widths by the generator coordinate method
- Description of the asymmetric to symmetric fission transition in the neutron-deficient Thoriums -- Role of the tensor force
- Generalized time-dependent generator coordinate method for small and large amplitude collective motion
- Spatial orientation of the fission fragment intrinsic spins and their correlations
- A dynamical model calculation to reconcile the nuclear fission lifetime from different measurement techniques
- Pairing dynamics and solitonic excitations in collisions of medium-mass, identical nuclei
- Properties of a quantum vortex in neutron matter
- Generation, dynamics, and correlations of the fission fragments' angular momenta
- Benchmark of the GEF model for fission-fragment yields over an enlarged range
- Pure quantum extension of the semiclassical Boltzmann-Uehling-Uhlenbeck equation
- Structures in the energy distribution of the scission neutrons: finite neutron-number effect
- Fission Fragment Excitation Energy Sharing Beyond Scission
- Nuclear Quantum Many-Body Dynamics: From Collective Vibrations to Heavy-Ion Collisions (2nd edition)
- Smoothing of one- and two-dimensional discontinuities in potential energy surfaces
- Decay widths at the scission point in nuclear fission
- Microscopic Calculation of Fission Product Yields for Odd-Mass Nuclei
- Superfluid extension of the self-consistent time-dependent band theory for neutron star matter: Anti-entrainment versus superfluid effects in the slab phase
- Manifestation of relative phase in dynamics of two interacting Bose-Bose droplets
- TDHF and a macroscopic aspect of low-energy nuclear reactions
- A schematic reaction-theory model for nuclear fission
- Fermionic Quantum Turbulence: Pushing the Limits of High-Performance Computing
- Correlations Between Fission Fragment and Neutron Anisotropies in Neutron-Induced Fission
- Experimental evidence of the effect of nuclear shells on fission dissipation and time
- Generator coordinate method for transition-state dynamics in nuclear fission
- Effects of the tensor force on low-energy heavy-ion fusion reactions: A mini review
- Solitonic excitations in collisions of superfluid nuclei: a qualitatively new phenomenon distinct from the Josephson effect
- Nuclear ground states in a consistent implementation of the time-dependent density matrix approach
- An implementation of nuclear time-dependent density-functional theory and its application to the nuclear isovector electric dipole resonance
- Time-dependent nuclear energy-density functional theory toolkit for neutron star crust: Dynamics of a nucleus in a neutron superfluid
- New developments in fission studies within the time-dependent density functional theory framework
- Sensitivity to the initial conditions of the Time-Dependent Density Functional Theory
- A microscopic model for spontaneous fission: validity of the adiabatic approximation
- Fission of relativistic nuclei with fragment excitation and reorientation
- Diabatic scission paths
- Time-dependent mean field determination of the excitation energy in transfer reactions: application to the reaction U on C at 6.14 MeV/A
- Time-dependent density functional theory study of induced-fission dynamics of Th
- The shapes of nuclei
- Non-Markovian character and irreversibility of real-time quantum many-body dynamics
- Microscopic collective inertial masses for nuclear reaction in the presence of nucleonic effective mass
- Time-Dependent Density Functional Theory Description of U(n,f), Pu(n,f) and Np(n,f) Reactions
- Pygmy resonances: what's in a name?
- Inertial energy dissipation in nuclear dynamics
- Pygmy resonances and symmetry energy
- Examining the justification for the introduction of a fermion localization function
- Nuclear Fission: from more phenomenology and adjusted parameters to more fundamental theory and increased predictive power
- Nuclear reaction path and requantization of TDDFT
- Microscopic theory of angular momentum distributions across the full range of fission fragments
- A microscopic calculation of fission cross sections with the non-equilibrium Green function method
- Continuum damping effects in nuclear collisions associated with twisted boundary conditions
- Non-Equilibrium Aspects of Fission Dynamics within the Time Dependent Density Functional Theory
- Fission in a microscopic framework: from basic science to support for applications
- Fragment Intrinsic Spins and Fragments' Relative Orbital Angular Momentum in Nuclear Fission
- A critical assessment of the current implementations of the Generator Coordinate Method
- Microscopic self-consistent description of induced fission: dynamical pairing degree of freedom
- Pigmy resonances, transfer, and separable potentials
- Microscopic Calculations of Vortex-Nucleus Interaction in the Neutron Star Crust
- The LISE package: solvers for static and time-dependent superfluid local density approximation equations in three dimensions
- Isotopic fission yields of Pu as a function of the excitation energy
- Microscopic Theory of Nuclear Fission
- Bremsstrahlung emission accompanying ternary fission of \isotope[252]{Cf}
- Time-dependent mean-field investigations of the quasifission process
- Local energy density functional for superfluid Fermi gases from effective field theory
- Nuclear structure and reaction with quantum shape fluctuation