Creep and flow of glasses: strain response linked to the spatial distribution of dynamical heterogeneities

Abstract

Mechanical properties are of central importance to materials sciences, in particular if they depend on external stimuli. Here we investigate the rheological response of amorphous solids, namely col- loidal glasses, to external forces. Using confocal microscopy and computer simulations, we establish a quantitative link between the macroscopic creep response and the microscopic single-particle dy- namics. We observe dynamical heterogeneities, namely regions of enhanced mobility, which remain localized in the creep regime, but grow for applied stresses leading to steady flow. These different behaviors are also reflected in the average particle dynamics, quantified by the mean squared dis- placement of the individual particles, and the fraction of active regions. Both microscopic quantities are found to be proportional to the macroscopic strain, despite the non-equilibrium and non-linear conditions during creep and the transient regime prior to steady flow.

10 pages, 6 figures

References in corpus (4)

• Three-dimensional imaging of colloidal glasses under steady shear
• Glass Rheology: From mode-coupling theory to a dynamical yield criterion
• Yielding of binary colloidal glasses
• Fluctuations and scaling in creep deformation

Cited by in corpus (5)

• Structure-property relationships via recovery rheology in viscoelastic materials
• Start-up Shear of Concentrated Colloidal Hard Spheres: Stresses, Dynamics and Structure
• Heterogeneous dynamics during yielding of glasses: effect of aging
• Triple junction at the triple point resolved on the individual particle level
• Plastic response and correlations in athermally sheared amorphous solids