Ultrafast flow of interacting organic polaritons
arXiv:1502.00602 · doi:10.1038/lsa.2016.212
Abstract
The strong-coupling of an excitonic transition with an electromagnetic mode results in composite quasi-particles called exciton-polaritons, which have been shown to combine the best properties of their bare components in semiconductor microcavities. However, the physics and applications of polariton flows in organic materials and at room temperature are still unexplored because of the poor photon confinement in such structures. Here we demonstrate that polaritons formed by the hybridization of organic excitons with a Bloch Surface Wave are able to propagate for hundreds of microns showing remarkable third-order nonlinear interactions upon high injection density. These findings pave the way for the studies of organic nonlinear light-matter fluxes and for a technological promising route of dissipation-less on-chip polariton devices working at room temperature.
Improved version with polariton-polariton interactions. 13 pages, 4 figures, supporting 6 pages, 6 figures
References in corpus (9)
- Observation of Superfluidity of Polaritons in Semiconductor Microcavities
- Quantised Vortices in an Exciton-Polariton Fluid
- Quantum-fluid dynamics of microcavity polaritons
- Extraordinary exciton conductance induced by strong coupling
- Cavity enhanced transport of excitons
- Control and ultrafast dynamics of a two-fluid polariton switch
- Realization of an all optical exciton-polariton router
- Slow reflection and two-photon generation of microcavity exciton-polaritons
- Polariton Induced Enhanced Emission from an Organic Dye under Strong Coupling Regime
Cited by in corpus (32)
- Room-temperature superfluidity in a polariton condensate
- Interacting polariton fluids in a monolayer of tungsten disulfide
- Unveiling the mixed nature of polaritonic transport: From enhanced diffusion to ballistic motion approaching the speed of light
- Ultrafast imaging of polariton propagation and interactions
- Tuning the coherent propagation of organic exciton-polaritons through dark state delocalization
- Dark state semilocalization of quantum emitters in a cavity
- Tailoring dispersion of room temperature exciton-polaritons with perovskite-based subwavelength metasurfaces
- Edge-emitting polariton laser and amplifier based on a ZnO waveguide
- Disorder-Enhanced and Disorder-Independent Transport with Long-Range Hopping: Application to Molecular Chains in Optical Cavities
- Polariton Localization and Dispersion Properties of Disordered Quantum Emitters in Multimode Microcavities
- Unusual Dynamical Properties of Disordered Polaritons in Micocavities
- Polariton-Enhanced Exciton Transport
- Engineering random spin models with atoms in a high-finesse cavity
- Disorder-enhanced transport in a chain of lossy dipoles strongly coupled to cavity photons
- Tuning the Coherent Propagation of Organic Exciton-Polaritons through the Cavity Q-factor
- Generation of Anti-Stokes Fluorescence in a Strongly Coupled Organic Semiconductor Microcavity
- Non-Hermitian molecular dynamics simulations of exciton-polaritons in lossy cavities
- Exciton-Polaritons in Uniaxially Aligned Organic Microcavities
- Theoretical Analysis of Exciton Wave Packet Dynamics in Polaritonic Wires
- Superluminal X-waves in a polariton quantum fluid
- Centimeter-scale propagation of optical surface waves at visible wavelengths
- Coherent transient exciton transport in disordered polaritonic wires
- Superpolynomial Quantum Enhancement in Polaritonic Neuromorphic Computing
- Polariton Hall Effect in Transition-Metal Dichalcogenides
- Photochemical Initiation of Polariton Propagation
- Transport regimes for exciton-polaritons in disordered microcavities
- Competition between horizontal and vertical polariton lasing in planar microcavities
- Disentangling enhanced diffusion and ballistic motion of excitons coupled to Bloch surface waves with molecular dynamics simulations
- Directional Flow of Confined Polaritons in CrSBr
- Nonlinear optical spectroscopy of open quantum systems
- Polariton transport in 2D semiconductors: Phonon-mediated transitions between ballistic, superdiffusive and exciton-limited regimes
- General theory of cavity-mediated interactions between low-energy matter excitations