Electromagnetic coupling of spins and pseudospins in bilayer graphene

Abstract

We present a detailed theoretical study of bilayer-graphene's electronic properties in the presence of electric and magnetic fields. Using group-theoretical methods, we derive an invariant expansion of the Hamiltonian for electron states near the K point of the Brillouin zone. In contrast to known materials, including single-layer graphene, any possible coupling of physical quantities to components of the external electric (magnetic) field has a counterpart where the analogous component of the magnetic (electric) field couples to exactly the same combination of quantities. For example, a purely electric spin splitting appears as the magneto-electric analogue of the familiar magnetic Zeeman spin splitting. The measurable thermodynamic response induced by magnetic and electric fields is thus completely symmetric. The Pauli magnetization induced by a magnetic field takes exactly the same functional form as the polarization induced by an electric field. Our findings thus reveal unconventional behavior of spin and pseudospin degrees of freedom in their coupling to external fields. We explain how these counterintuitive couplings are consistent with fundamental principles such as time reversal symmetry. For example, only a magnetic field can give rise to a macroscopic spin polarization, whereas only a perpendicular electric field can induce a macroscopic polarization of the sublattice-related pseudospin degree of freedom characterizing the intravalley orbital motion in bilayer graphene. These rules enforced by symmetry for the matter-field interactions clarify the nature of spins versus pseudospins. We also provide numerical values of prefactors for relevant coupling terms. While our theoretical arguments use bilayer graphene as an example, they are generally valid for any material with similar symmetries.

15 pages, 2 figures. revised final version, supersedes arXiv:1206.4761

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• Topological Field Theory of Time-Reversal Invariant Insulators
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• Asymmetry gap in the electronic band structure of bilayer graphene
• The electronic properties of bilayer graphene
• Relativistic analysis of magnetoelectric crystals: extracting a new 4-dimensional P odd and T odd pseudoscalar from Cr_2 O_3 data
• Magnetoelectric effect in bilayer graphene controlled by valley-isospin density