Theory of field-induced quantum phase transition in spin dimer system BaCrO
arXiv:1405.0564 · doi:10.1016/j.jmmm.2014.01.045
Abstract
Motivated by recent experiments on BaCrO, we propose a theory describing low-temperature properties in magnetic field of dimer spin- systems on a stacked triangular lattice with spatially anisotropic exchange interactions. Considering the interdimer interaction as a perturbation we derive in the second order the elementary excitations (triplon) spectrum and the effective interaction between triplons at the quantum critical point separating the paramagnetic phase () and a magnetically ordered one (, where is the saturation field). Expressions are derived for and the staggered magnetization at close to . We apply the theory to BaCrO and determine exchange constants of the model by fitting the triplon spectrum obtained experimentally. It is demonstrated that in accordance with experimental data the system follows the 3D BEC scenario at K only due to a pronounced anisotropy of the spectrum near its minimum. Our expressions for , and fit well available experimental data.
arXiv comment9 pages, 6 figures
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