Magnetic order and spin dynamics in La2O2Fe2OSe2 probed by 57Fe-Moessbauer, 139La-NMR, and muon spin relaxation spectroscopy

Abstract

We present a detailed local probe study of the magnetic order in the oxychalcogenide La2O2Fe2OSe2 utilizing 57Fe Moessbauer, 139La NMR, and muon spin relaxation spectroscopy. This system can be regarded as an insulating reference system of the Fe arsenide and chalcogenide superconductors. From the combination of the local probe techniques we identify a non-collinear magnetic structure similar to Sr2F2Fe2OS2. The analysis of the magnetic order parameter yields an ordering temperature TN = 90.1 K and a critical exponent of beta = 0.133, which is close to the 2D Ising universality class as reported in the related oxychalcogenide family.

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• Magnetic and Structural Properties of the Iron Oxychalcogenides La${}_2$O${}_2$Fe${}_2$O$M_2$ ($M$= S, Se)
• Strong charge and spin fluctuations in La${}_2$O${}_3$Fe${}_2$Se${}_2$
• Local Structure of Mott Insulating Iron Oxychalcogenides La${}_2$O${}_2$Fe${}_2$O$M$${}_2$ ($M$ = S, Se)
• Crystal field excitations and magnons: their roles in oxyselenides Pr2O2M2OSe2 (M = Mn, Fe)
• Impact of disorder on dynamics and ordering in the honeycomb lattice iridate Na${}_2$IrO${}_3$
• Chemistry and physics of layered oxychalcogenides containing an anti-cuprate type square lattice
• Magnetically-induced local lattice anomalies and low-frequency nematic fluctuations in the Mott insulator La${}_2$O${}_3$Fe${}_2$Se${}_2$