Electronics with correlated oxides: SrVO/SrTiO as a Mott transistor
arXiv:1312.5989 · doi:10.1103/PhysRevLett.114.246401
Abstract
We employ density functional theory plus dynamical mean field theory and identify the physical origin of why two layers of SrVO on a SrTiO substrate are insulating: the thin film geometry lifts the orbital degeneracy which in turn triggers a Mott-Hubbard transition. Two layers of SrVO are just at the verge of a Mott-Hubbard transition and hence ideally suited for technological applications of the Mott-Hubbard transition: the heterostructure is highly sensitive to strain, electric field, and temperature. A gate voltage can also turn the insulator into a metal, so that a transistor with ideal on-off (metal-insulator) switching properties is realized.
References in corpus (16)
- Continuous-time Monte Carlo methods for quantum impurity models
- Electric Field Control of the LaAlO/SrTiO Interface Ground State
- Screened Coulomb interaction in the maximally localized Wannier basis
- Kinks in the dispersion of strongly correlated electrons
- Enhanced Crystal Field Splitting and Orbital Selective Coherence by Strong Correlations in V_2O_3
- Antiferromagnetic Order of Strongly Interacting Fermions in a Trap: Real-Space Dynamical Mean-Field Analysis
- Momentum-resolved spectral functions of SrVO calculated by LDA+DMFT
- Oxide Heterostructures for Efficient Solar Cells
- Resistive switching induced by electronic avalanche breakdown in GaTaSeTe narrow gap Mott Insulators
- Combined GW and dynamical mean field theory: Dynamical screening effects in transition metal oxides
- Conserved quantities of SU(2)-invariant interactions for correlated fermions and the advantages for quantum Monte Carlo simulations
- Dynamical vertex approximation for nanoscopic systems
- Importance of d-p Coulomb interaction for high T cuprates and other oxides
- Optical Properties of Correlated Materials -- or Why Intelligent Windows may look Dirty
- Effective Coulomb interactions in solids under pressure
- Nanoscale Dynamical Mean-Field Theory for Molecules and Mesoscopic Devices in the Strong-Correlation Regime
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- Nano-engineering of electron correlation in oxide superlattices
- An electric-field driven Mott metal-insulator transition in correlated thin films: an inhomogeneous dynamical mean-field theory approach
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- Multilayer engineering of CaVO thin films with SrTiO and LaAlO from DFT+DMFT
- Charge self-consistent density functional theory plus ghost rotationally-invariant slave-boson theory for correlated materials
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- Mixed-configuration approximation for multiorbital systems out of equilibrium
- Quantified Degeneracy, Entropy and Metal-Insulator Transition in Complex Transition-Metal Oxides
- Photoemission and Dynamical Mean Field Theory Study of Electronic Correlation in a Metal of SrRhO Thin Film
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