Antiferromagnetic Order and Superconductivity in Sr4(Mg0.5-xTi0.5+x)2O6Fe2As2 with Electron Doping: 75As-NMR Study

Abstract

We report an 75As-NMR study on iron (Fe)-based superconductors with thick perovskitetype blocking layers Sr4(Mg0.5-xTi0.5+x)2O6Fe2As2 with x=0 and 0.2. We have found that antiferromagnetic (AFM) order takes place when x=0, and superconductivity (SC) emerges below Tc=36 K when x=0.2. These results reveal that the Fe-pnictides with thick perovskitetype blocks also undergo an evolution from the AFM order to the SC by doping electron carriers into FeAs planes through the chemical substitution of Ti+4 ions for Mg+2 ions, analogous to the F-substitution in LaFeAsO compound. The reason why the Tc=36 K when x=0.2 being higher than the optimally electron-doped LaFeAsO with Tc=27 K relates to the fact that the local tetrahedron structure of FeAs4 is optimized for the onset of SC.

arXiv comment4 pages, 3 figures, 1 table

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• NMR evidence for an intimate relationship between antiferromagnetic spin fluctuations and extended s-wave superconductivity in mono-crystalline SrFe2(As_{1-x}P_{x})2
• High-Tc Nodeless s_\pm-wave Superconductivity in (Y,La)FeAsO_{1-y} with Tc=50 K: 75As-NMR Study
• NMR Investigation of the iron-based superconductors Ca4(Mg,Ti)3Fe2As2O8-y and Ca5(Sc,Ti)4Fe2As2O11-y
• High-$T_c$ Iron-phosphide Superconductivity Enhanced by Reemergent Antiferromagnetic Spin Fluctuations in (Sr${}_4$Sc${}_2$O${}_6$)Fe${}_2$(As${}_{1-x}$P${}_x$)${}_2$ probed by NMR
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