The metallic transport of (TMTSF)_2X organic conductors close to the superconducting phase
arXiv:1105.3323 · doi:10.1088/0953-8984/23/34/345702
Abstract
Comparing resistivity data of quasi-one dimensional superconductors (TMTSF)_2PF_6 and (TMTSF)_2ClO_4 along the least conducting c*-axis and along the high conductivity a -axis as a function of temperature and pressure, a low temperature regime is observed in which a unique scattering time governs transport along both directions of these anisotropic conductors. However, the pressure dependence of the anisotropy implies a large pressure dependence of the interlayer coupling. This is in agreement with the results of first-principles DFT calculations implying methyl group hyperconjugation in the TMTSF molecule. In this low temperature regime, both materials exhibit for rc a temperature dependence aT + bT^2. Taking into account the strong pressure dependence of the anisotropy, the T-linear rc is found to correlate with the suppression of the superconducting Tc, in close analogy with ra data. This work is revealing the domain of existence of the 3D coherent regime in the generic (TMTSF)_2X phase diagram and provides further support for the correlation between T-linear resistivity and superconductivity in non-conventional superconductors.
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- Crossover from impurity-controlled to granular superconductivity in (TMTSF)2ClO4
- Novel superconducting phenomena in quasi-one-dimensional Bechgaard salts
- Quasi one-dimensional organic conductors: from Fröhlich conductivity and Peierls insulating state to magnetically-mediated superconductivity, a retrospective
- Evolution of shape and volume fraction of superconducting domains with temperature and anion disorder in (TMTSF)ClO
- Influence of carrier lifetime on quantum criticality and superconducting Tc of (TMTSF)_2ClO_4