Transient localization in crystalline organic semiconductors
arXiv:1010.2893 · doi:10.1103/PhysRevB.83.081202
Abstract
A relation derived from the Kubo formula shows that optical conductivity measurements below the gap frequency in doped semiconductors can be used to probe directly the time-dependent quantum dynamics of charge carriers. This allows to extract fundamental quantities such as the elastic and inelastic scattering rates, as well as the localization length in disordered systems. When applied to crystalline organic semiconductors, an incipient electron localization caused by large dynamical lattice disorder is unveiled, implying a breakdown of semiclassical transport.
Revised version, to appear in Phys. Rev. B Rapid Communications
References in corpus (4)
Cited by in corpus (50)
- The transient localization scenario for charge transport in crystalline organic materials
- Coherent quantum transport in disordered systems I: The influence of dephasing on the transport properties and absorption spectra on one-dimensional systems
- Linear Scaling Quantum Transport Methodologies
- A General Charge Transport Picture for Organic Semiconductors with Nonlocal Electron-Phonon Couplings
- Coherent quantum transport in disordered systems: A unified polaron treatment of hopping and band-like transport
- Conductivity of graphene with resonant and non-resonant adsorbates
- Electronic transport and quantum localization effects in organic semiconductors
- Band dispersion and electronic lifetimes in crystalline organic semiconductors
- A unification of the Holstein polaron and dynamic disorder pictures of charge transport in organic semiconductors
- Finite Temperature TD-DMRG for the Carrier Mobility of Organic Semiconductors
- Modelization of charge carriers mobilities in halide perovskites: Fröhlich scattering and quantum localization effects in a dynamic disorder regime
- Phenomenological model for charge dynamics and optical response of disordered systems: application to organic semiconductors
- On dynamical localization corrections to band transport
- Crossover from Super- to Sub-Diffusive Motion and Memory Effects in Crystalline Organic Semiconductors
- Intermediate Polaronic Charge Transport in Organic Crystals from a Many-Body First-Principles Approach
- Electronic properties of asymmetrically doped twisted graphene bilayers
- Monte Carlo simulation based on dynamic disorder model in organic semiconductors: From bandlike to hopping transport
- Displaced Drude peak and bad metal from the interaction with slow fluctuations
- Combining linear-scaling quantum transport and machine-learning molecular dynamics to study thermal and electronic transports in complex materials
- Optical conductivity and optical effective mass in a high-mobility organic semiconductor: Implications for the nature of charge transport
- Coherent charge carrier dynamics in the presence of thermal lattice vibrations
- Transient localization from the interaction with quantum bosons
- A spin-boson theory for charge photogeneration in organic molecules: Role of quantum coherence
- Drift of Charge Carriers in Crystalline Organic Semiconductors
- Anomalous electronic transport in Quasicrystals and related Complex Metallic Alloys
- Decoherence and Energy Relaxation in the Quantum-Classical Dynamics for Charge Transport in Organic Semiconducting Crystals: an Instantaneous Decoherence Correction Approach
- Understanding the correlation between electronic coupling and energetic stability of molecular crystal polymorphs: The instructive case of quinacridone
- Quantum acoustics unravels Planckian resistivity
- First-principle quantum Monte-Carlo study of charge carrier mobility in organic molecular semiconductors
- Charge transport limited by nonlocal electron-phonon interaction. II. Numerically exact quantum dynamics in the slow-phonon regime
- Precursors to Anderson Localization in the Holstein Model: Quantum and Quantum-Classical Solutions
- Conductivity of an electron coupled to anharmonic phonons
- Dynamical quantum typicality: Simple method for investigating transport properties applied to the Holstein model
- Charge transport limited by nonlocal electron-phonon interaction. I. Hierarchical equations of motion approach
- Polaronic quantum diffusion in dynamic localization regime
- Efficient Time-Domain Approach for Linear Response Functions
- Two-dimensional electronic transport in rubrene: the impact of inter-chain coupling
- Diagrammatic quantum Monte Carlo toward the calculation of transport properties in disordered semiconductors
- Dissecting Exciton-Polariton Transport in Organic Molecular Crystals: Emerging Conductivity Assisted by Intermolecular Vibrational Coupling
- Strategies for controlling through-space charge transport in metal-organic frameworks via structural modifications
- Modeling Nonlocal Electron-Phonon Coupling in Organic Crystals Using Interpolative Maps: The Spectroscopy of Crystalline Pentacene and 7,8,15,16-Tetraazaterrylene
- Two channel model for optical conductivity of high mobility organic crystals
- Electronic structure and transport in materials with flat bands: 2D materials and quasicrystals
- Investigating electron conductivity regimes in the bacterial cytochrome wire OmcS
- Polaron catastrophe within quantum acoustics
- Numerically "exact" charge transport dynamics in a dissipative electron-phonon model rationalizing the success of the transient localization scenario
- Localization and spectrum of quasiparticles in a disordered fermionic Dicke model
- Non-equilibrium Optical Conductivity in Materials with Localized Electronic States
- Quantum-classical study of charge transport in organic semiconductors with multiple low-frequency vibrational modes
- Path-Integral Approach to Quantum Acoustics