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Ultrafast Coherence Delocalization in Real Space Simulated by Polaritons
Bo Xiang, Zimo Yang, Yi-Zhuang You +1
We investigated coherence delocalization on a coupled-cavity molecular polariton platform in time, frequency, and spatial domains, enabled by ultrafast two-dimensional infrared hyp…
Theory for Nonlinear Spectroscopy of Vibrational Polaritons
Raphael F. Ribeiro, Adam D. Dunkelberger, Bo Xiang +4
Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent exp…
Revealing Hidden Vibration Polariton Interactions by 2D IR Spectroscopy
Bo Xiang, Raphael F. Ribeiro, Adam D. Dunkelberger +6
We report the first experimental two-dimensional infrared (2D IR) spectra of novel molecular photonic excitations - vibrational-polaritons. The application of advanced 2D IR spectr…