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Full-wave nonlinear microscopy reveals guided channel for ultrafast polariton transport
Qingyi Zhou, Piper Fowler-Wright, Zongfu Yu +2
We show how finite-difference time-domain (FDTD) simulations can be extended to model ultrafast nonlinear microscopy, enabling the prediction of spatially-resolved pump--probe sign…
Mapping molecular polariton transport via pump-probe microscopy
Piper Fowler-Wright, Michael Reitz, Joel Yuen-Zhou
We demonstrate how the transport properties of molecular polaritons in optical cavities can be extracted from a microscopic modeling of pump-probe spectroscopy. Our approach combin…
Multidimensional semiclassical single- and double-quantum spectroscopy of anharmonic molecular polaritons
Michael Reitz, Harsh Bhakta, Wei Xiong +1
We present a general and efficient approach to compute phase-resolved multidimensional spectra of anharmonic molecular polaritons, based on a semiclassical evolution of the molecul…
Permutationally symmetric molecular aggregates
Sricharan Raghavan-Chitra, Arghadip Koner, Joel Yuen-Zhou
Linear optical spectra of molecular aggregates are often approximated by classical optics methods such as the discrete-dipole approximation (DDA), coherent exciton scattering (CES)…
Quantum theory of surface lattice resonances
Michael Reitz, Stephan van den Wildenberg, Arghadip Koner +2
The collective interactions of nanoparticles arranged in periodic structures give rise to high- in-plane diffractive modes known as surface lattice resonances. While these reson…
Exploring the Delocalization of Dark States in a Multimode Optical Cavity
Kunyang Sun, Matthew Du, Joel Yuen-Zhou
The strong coupling between molecules and photonic modes in a Fabry-Pérot optical cavity, which forms hybrid light-matter states called polaritons, has been demonstrated as a prom…