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physics.chem-ph2023
Singlet Fission in Lycopene H-Aggregates
William Barford
A theory of singlet fission (SF) in carotenoid dimers is applied to explain the SF in lycopene H-aggregates observed after high energy photoexcitation. The explanation proposed her…
physics.chem-ph2023
Theory of Singlet Fission in Carotenoid Dimers
William Barford, Cameron A Chambers
We develop a theory of singlet fission in carotenoid dimers. Following photoexcitation of the 'bright' state (i.e., a singlet electron-hole pair) in a single carotenoid, the first…