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Nonlinear rotational spectroscopy reveals many-body interactions in water molecules
Yaqing Zhang, Jiaojian Shi, Xian Li +3
Because of their central importance in chemistry and biology, water molecules have been the subject of decades of intense spectroscopic investigations. Rotational spectroscopy of w…
Rapid and Precise Determination of Zero-Field Splittings by Terahertz Time-Domain Electron Paramagnetic Resonance Spectroscopy
Jian Lu, I. Ozge Ozel, Carina Belvin +7
Zero-field splitting (ZFS) parameters are fundamentally tied to the geometries of metal ion complexes. Despite their critical importance for understanding the magnetism and spectro…
How two-dimensional brick layer J-aggregates differ from linear ones: excitonic properties and line broadening mechanisms
Arend G. Dijkstra, Hong-Guang Duan, Jasper Knoester +2
We study the excitonic coupling and homogeneous spectral line width of brick layer J-aggregate films. We begin by analysing the structural information revealed by the two-exciton s…
Molecular Orientation by Intense Single Cycle THz Pulses
Sharly Fleischer, Yan Zhou, Robert W. Field +1
Intense single-cycle THz pulses resonantly interacting with molecular rotations are shown to induce significant field-free orientation under ambient conditions. We calculate and me…