activity
20102026
most citedOrigin of Long Lived Coherences in Light-Harvesting Complexes

402 citations · 1.2k across the 30 of their papers we have counts for

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Showing 2010Show all

6 papers · 1 filter

quant-ph2010

Quantum Master Equations for Non-linear Optical Response of Molecular Systems

Tomas Mancal, Frantisek Sanda

Generalized master equations valid for the third order response of an optically driven multi-level electronic system are derived within Zwanzig projection formalism. Each of three…

physics.chem-ph2010★ 58 cited

Vibrational wave packet induced oscillations in two-dimensional electronic spectra. II. Theory

Tomas Mancal, Alexandra Nemeth, Franz Milota +3

We present a theory of vibrational modulation of two-dimensional coherent Fourier transformed electronic spectra. Based on an expansion of the system's energy gap correlation funct…

physics.chem-ph2010★ 64 cited

Vibrational wave packet induced oscillations in two-dimensional electronic spectra. I. Experiments

Alexandra Nemeth, Franz Milota, Tomas Mancal +4

This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series…

physics.chem-ph2010★ 15 cited

Decoherence in Weakly Coupled Excitonic Complexes

Tomas Mancal, Vytautas Balevicius, Leonas Valkunas

Equations of motion for weakly coupled excitonic complexes are derived. The description allows to treat the system in the basis of electronic states localized on individual chromop…

physics.bio-ph2010★ 103 cited

Exciton Dynamics in Photosynthetic Complexes: Excitation by Coherent and Incoherent Light

Tomas Mancal, Leonas Valkunas

In this paper we consider dynamics of a molecular system subjected to external pumping by a light source. Within a completely quantum mechanical treatment, we derive a general form…

physics.chem-ph2010★ 13 cited

Electronic Coherence Dephasing in Excitonic Molecular Complexes: Role of Markov and Secular Approximations

Jan Olsina, Tomas Mancal

We compare four different types of equations of motion for reduced density matrix of a system of molecular excitons interacting with thermodynamic bath. All four equations are of s…